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Record W4405513202 · doi:10.1016/j.mineng.2024.109157

Leaching and recovery of rare earth elements, copper, nickel, silver and gold from used smartphone circuit boards

2024· article· en· W4405513202 on OpenAlexafffund
Salmata Diallo, Lan Huong Tran, Dominic Larivière, Jean-François Blais

Bibliographic record

VenueMinerals Engineering · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicRecycling and Waste Management Techniques
Canadian institutionsUniversité LavalInstitut National de la Recherche Scientifique
FundersFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of Canada
KeywordsLeaching (pedology)NickelRare earthMetallurgyCopperPrinted circuit boardMaterials scienceEnvironmental scienceEngineeringElectrical engineering

Abstract

fetched live from OpenAlex

Printed circuit board (PCB) assemblies constitute a concentrated source of valuable metals. This study evaluates the performance of a complete hydrometallurgical process for extracting and recovering rare earth elements (REE), Cu, Ni, Ag and Au from leachates produced from PCB found in smartphones via four selective leaching steps. In a REE leachate ([Dy] = 43 mg/L, [Gd] = 5 mg/L, [Nd] = 266 mg/L, [Sm] = 35 mg/L, [Tb] = 8 mg/L, [Ho] = 2 mg/L), 92 % of REE was precipitated at room temperature with H 2 C 2 O 4 /REE molar ratio of 2/1. Calcination of the REE-oxalate precipitates at 800 °C resulted in a mixture of rare earth oxides (REO) with a 91 % purity. From the base metal leachate ([Cu] = 19,376 mg/L and [Ni] = 1,264 mg/L), Cu was electrodeposited during 120 min (pH = 3, current 270 A/m 2 ) while Ni was precipitated by addition of oxalic acid (H 2 C 2 O 4 /Ni molar ratio of 2/1, pH 4.4, T = 60 °C, t = 60 min), followed by calcination at 600 °C for 4 h to form NiO (93 % purity). Three oxidative leaching steps (10 % w/v solids, T = 80 °C, t = 180 min, 1.0 M H 2 SO 4 , 67 g H 2 O 2 /L, T = 80 °C, t = 180 min) solubilized 97 % of Ag. Subsequently, with the addition of Cu (Cu/Ag mass ratio of 2), at room temperature and 120 min, Ag was precipitated 99.4 % in the first leachate ([Ag] = 488 mg/L). A Zn/Au mass ratio of 30 precipitated 99.1 % of gold at the room-temperature from the gold leachate ([Au] = 107 mg/L).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.731
Threshold uncertainty score0.560

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.205
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2024
Admission routes2
Has abstractyes

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