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Record W4405675501 · doi:10.1002/adma.202416375

Two‐dimensional Nanosheets by Liquid Metal Exfoliation

2024· article· en· W4405675501 on OpenAlexaff
Yichao Bai, Youan Xu, Linxuan Sun, Zack Ward, Hongzhang Wang, Gothamie Ratnayake, Cong Wang, Mingchuang Zhao, Haoqi He, Jianxiang Gao, Menghan Wu, Sirong Lu, George Bepete, Deli Peng, Bilu Liu, Feiyu Kang, Humberto Terrones, Mauricio Terrones, Yu Lei

Bibliographic record

VenueAdvanced Materials · 2024
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsConcordia University
FundersNational Science Fund for Distinguished Young ScholarsNational Key Research and Development Program of ChinaNational Natural Science Foundation of China
KeywordsMaterials scienceExfoliation jointIntercalation (chemistry)van der Waals forceSurface tensionGalliumGrapheneChemical engineeringDispersion (optics)Phase (matter)NanotechnologyMetalPulmonary surfactantBirefringenceMoleculeInorganic chemistryOpticsOrganic chemistryMetallurgy

Abstract

fetched live from OpenAlex

Abstract Liquid exfoliation is a scalable and effective method for synthesizing 2D nanosheets (NSs) but often induces contamination and defects. Here, liquid metal gallium (Ga) is used to exfoliate bulk layered materials into 2D NSs at near room temperature, utilizing the liquid surface tension and Ga intercalation to disrupt Van der Waals (vdW) forces. In addition, the process can transform the 2H‐phase of transition metal dichalcogenides into the 1T’‐phase under ambient conditions. This method produces high aspect ratio, surfactant‐free 2D‐NSs for more than 10 types of 2D materials that include h‐BN, graphene, MoTe 2 , MoSe 2 , layered minerals, etc. The subsequent Ga separation via ethanol dispersion avoids the formation of additional defects and surfactant contamination. By adjusting initial defect levels of the layered materials, customize the metallicity and/or defectiveness of 2D NSs can be customized for applications such as birefringence‐tunable modulators with exfoliated h‐BN, and enhanced hydrogen evolution with defective MoS 2 . This approach offers a strategy to optimize liquid metal/2D interfaces, preserving intrinsic properties and enabling practical applications, potentially transforming optics, energy conversion, and beyond.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.032
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.281
Teacher spread0.271 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2024
Admission routes1
Has abstractyes

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