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Record W4405988464 · doi:10.1016/j.clay.2024.107693

PEO flocculation of kaolinite – Molecular weight effect

2025· article· en· W4405988464 on OpenAlexafffund
Chao Deng, Daowei Wang, Gen Huang, Jihui Li, Zeyang Xu, Liqiang Ma, Qi Liu

Bibliographic record

VenueApplied Clay Science · 2025
Typearticle
Languageen
FieldMaterials Science
TopicClay minerals and soil interactions
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship Council
KeywordsKaoliniteFlocculationChemical engineeringChemistryMaterials scienceGeologyMineralogyGeochemistryOrganic chemistry

Abstract

fetched live from OpenAlex

The adsorption of poly(ethylene oxide) (PEO) of different molecular weights (MW) on kaolinite and its effects on kaolinite suspension stability were investigated. Fourier transform infrared spectroscopic and X-ray photoelectron spectroscopic analyses showed that the adsorption mechanisms of PEOs with different molecular weights appeared to be identical, i.e., through the formation of hydrogen bonds between ether‑oxygen groups of PEO and hydroxyl groups on the surface of kaolinite. Zeta potential measurements indicated that the adsorption of PEO resulted in the outward expansion of the diffuse layer on the surface of kaolinite, as evidenced by a decrease in the magnitude of zeta potential. The maximum decrease was observed to correlate to the thickness of the adsorbed layer, which in turn was proportional to the MW of PEO, indicative of the lateral extension of the “loop” and “tail” structures of adsorbed PEO. As the adsorption layer thickness increased, the likelihood of bridging flocculation increased, resulting in the formation of larger flocs with greater strength and lower density in a shorter time, observed with higher MW PEO. This conclusion was confirmed by experimental results obtained from an online monitoring system for flocculation processes composed of focused beam reflectance measurement (FBRM) particle size analyzer and confocal scanning microscopy (CSM).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.277
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2025
Admission routes2
Has abstractyes

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