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Record W4406325143 · doi:10.1021/acsaelm.4c01396

Correlation between Material Properties, Crystalline Transitions, and Point Defects in RF Sputtered (N,Mg)-Doped Copper Oxide Thin Films

2025· article· en· W4406325143 on OpenAlex
Thomas Ratz, Emile Fourneau, Naama Sliti, Cédric Malherbe, Amaury Baret, Bénédicte Vertruyen, A. V. Silhanek, Ngoc Duy Nguyen

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Applied Electronic Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicCopper-based nanomaterials and applications
Canadian institutionsIONICS Mass Spectrometry (Canada)
FundersFonds Wetenschappelijk OnderzoekFonds De La Recherche Scientifique - FNRS
KeywordsMaterials scienceDopingThin filmCopperOxideCopper oxideOptoelectronicsMetallurgyNanotechnology

Abstract

fetched live from OpenAlex

In the present work, we investigate the effects of N and Mg doping on the optical and electrical properties of Cu 2 O thin films deposited using radiofrequency magnetron sputtering at room temperature. Additionally, crystalline phases are studied through complementary X-ray diffraction and energy dispersive X-ray spectroscopy measurements. It is shown that nitrogen incorporation enhances both the electrical and optical properties, with resistivity reaching a value as low as 1.15 Ωcm and an average transmittance in the visible range of 31.74%. Raman spectroscopy measurements indicate an increase in the number of (N 2 ) Cu shallow acceptor point defects, explaining the probed enhancement of p-type majority charge carriers. Also, in Mg-doped samples, marginal improvement of the optoelectrical properties is established. Conversely, we demonstrate that co-doping with Mg and N degrades the material crystallinity, leading to a reduction of thin film conductivity that could be attributed to high nitrogen incorporation. Subsequently, the influence of dopants on the electrical and optical properties is discussed via the analysis of the correlation between defects and Raman activities in the studied copper oxide thin films. This work contributes to the assessment of Mg and N as doping species, unveiling the dominant behavior of specific point defects. The results obtained in the study can therefore benefit future developments in copper-based p-type semiconducting oxides with enhanced optical and electrical properties.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.224
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it