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Record W4406949675 · doi:10.1021/acsapm.5c00076

Different Effect of Two Commonly Used Stearate Acid Scavengers on Polypropylene Crystallization Promotion Performance of a Sorbitol-Type Nucleating Agent

2025· article· en· W4406949675 on OpenAlexaff
Xinrao Zhang, Fushan Wang, Shiyuan Yang, Guangquan Li, Jiachun Feng

Bibliographic record

VenueACS Applied Polymer Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicPolymer crystallization and properties
Canadian institutionsPetro-Canada
FundersNational Natural Science Foundation of China
KeywordsSorbitolCrystallizationPolypropyleneStearatePromotion (chess)NucleationChemistryChemical engineeringMaterials scienceFood scienceOrganic chemistryPolitical scienceEngineering

Abstract

fetched live from OpenAlex

For Zieglar–Natta (Z–N) polypropylene (PP) to which a nucleating agent (NA) was added to regulate the properties, selecting an appropriate acid scavenger, a necessary additive for Z–N PP, is important for optimizing the effectiveness of the NA. However, the impact of various acid scavengers on the performance of NAs has not been systematically studied. In this work, the effect of two most widely used acid scavengers, calcium stearate (CaSt 2 ) and zinc stearate (ZnSt 2 ), on PP crystallization promotion performance of a commonly used NAs, NX8000 (a typical representative of sorbitol-type NAs family) was systematically investigated. It was found that CaSt 2 did not significantly alter the crystallization temperature ( T c ) of PP containing NX8000, while ZnSt 2 was detrimental to the nucleation benefit of NX8000, especially in the NA concentration range, where effective nucleation began but remained below the “critical saturation concentration”. The mechanism study showed that CaSt 2 added to PP almost remains chemically unchanged during heating and exhibits no significant impact on the NA. Differently, ZnSt 2 undergoes chemical reactions in a matrix at elevated temperature, producing stearic anhydride, which reacts with NX8000. As a result, a portion of the NA is consumed, leading to a reduction in its efficacy. Our work not only contributes to a comprehensive understanding of mechanisms when multiple additives are used simultaneously but also helps optimize additive formulations to maximize the performance of each component.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.256
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes1
Has abstractyes

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