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Record W4407247540 · doi:10.1021/acs.estlett.4c01126

Target and Suspect Screening Reveal PFAS Exceeding European Union Guideline in Various Water Sources South of Lyon, France

2025· article· en· W4407247540 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnvironmental Science & Technology Letters · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicPer- and polyfluoroalkyl substances research
Canadian institutionsUniversité de Montréal
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsTap waterContaminationEnvironmental chemistryEffluentEuropean unionEnvironmental scienceSurface waterGroundwaterChemistryEnvironmental engineeringGeology

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Lyon, a major hub for chemical industries in France, has been identified as a contamination hotspot of per- and polyfluoroalkyl substances (PFAS). Major chemical companies in the Pierre-Bénite area have used PFAS in the production of fluoropolymers and fluorotelomers, with effluents discharged into the Rhône River. This together with other contamination sources, such as firefighting foam use at a vicinal harbor oil depot, likely resulted in a complex PFAS signature. This study investigated PFAS contamination in various water sources in southern Lyon, including ponds, rivers, factory channels, wells, springs, and tap water. Out of 47 samples, 22 had a Σ 77 PFAS above 100 ng/L (maximum: ∼700 ng/L), and 67% of the tap water samples exceeded the European guideline of 100 ng/L for Σ 20 PFAS. Target PFAS profiles were dominated by perfluoroalkyl carboxylates (particularly C4 to C8), in agreement with their historical or current industrial usage. Suspect screening also revealed the occurrence of electrochemical fluorination precursors such as N-sulfopropyldimethylammoniopropyl perfluorohexanesulfonamido acetic acid (N-SPAmP-FHxSAA) and bistriflimide (used in the composition of ionic liquids). Certain fluorotelomers, including ESI+ (e.g., 6:2 fluorotelomer sulfonamidopropyl betaine (6:2 FTAB)) and ESI- (e.g., 6:2 FTS, 6:2 FTSAS-sulfone) compounds, were more prevalent in surface water than in tap or groundwater.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.167
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.004
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.218
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it