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Record W4407384089 · doi:10.1002/cjce.25615

Analysis of biomass as a feedstock in a chemical looping‐based polygeneration process for <scp>CO<sub>2</sub></scp> valorization

2025· article· en· W4407384089 on OpenAlexvenueno aff
Nimish Pankhedkar, S. N. Agnimitra Sunkara, Abhishek Dwivedi, Ravindra D. Gudi, Pratim Biswas, Suresh K. Bhargava

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2025
Typearticle
Languageen
FieldEngineering
TopicChemical Looping and Thermochemical Processes
Canadian institutionsnot available
Fundersnot available
KeywordsRaw materialBiomass (ecology)Process (computing)Waste managementEnvironmental scienceProcess engineeringPulp and paper industryEngineeringChemistryComputer science

Abstract

fetched live from OpenAlex

Abstract From the viewpoint of circular economy, the utilization of biomass as a preferred feedstock for power generation with carbon capture has become prevalent. Biomass utilization leads to a carbon‐neutral balance by leveraging its inherent carbon that was absorbed from the atmosphere. While chemical looping combustion (CLC) is a promising carbon capture technology for solid fuels such as coal, this paper further explores the feasibility of using biomass in CLC along with valorization of CO 2 to valuable chemicals. A polygeneration approach utilizing biomass has been proposed to produce power and value‐added chemicals (methanol and dimethyl ether [DME]), thus yielding an integrated CO 2 capture and utilization system. Biomass has a significant amount of oxygen and a higher H:C ratio than conventional fuels like coal. The effect of the same has been analyzed by assessing biomass as a feedstock in the proposed process and evaluating the effect of higher oxygen content towards the objective of CO 2 valorization relative to that of coal. Furthermore, a comparative discussion of the suitability of biomass compared to coal from a valorization perspective has been presented. Detailed techno‐feasibility analysis on the schemes and optimization studies to maximize the performance of the system in terms of energetics, CO 2 mitigation, and profitability has been conducted. From the analysis, it has been identified that the utilization of biomass as a feedstock in CLC‐based processes results in higher chemical production rates and higher profits with lesser CO 2 emissions than coal. The above analysis and evaluation has been carried out through simulations using Aspen Plus® software.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score0.787

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.218
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical EngineeringSame topicChemical Looping and Thermochemical ProcessesFrench-language works237,207