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Hydrogen uptake and embrittlement behavior in pipeline steels: Insights from slow strain rate testing and synchrotron micro-CT imaging

2025· article· en· W4407598368 on OpenAlexafffund
Tonye Alaso Jack, M. Adam Webb, K.M. Mostafijur Rahman, Fateh Fazeli, Jerzy A. Szpunar

Bibliographic record

VenueEngineering Failure Analysis · 2025
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen embrittlement and corrosion behaviors in metals
Canadian institutionsNatural Resources CanadaCanadian Light Source (Canada)University of Saskatchewan
FundersGovernment of SaskatchewanNatural Sciences and Engineering Research Council of CanadaNational Research CouncilCanadian Institutes of Health ResearchCanada Foundation for InnovationUniversity of Saskatchewan
KeywordsHydrogen embrittlementMaterials scienceSynchrotronStrain rateMetallurgyEmbrittlementPipeline (software)HydrogenStrain (injury)CorrosionEngineeringMedicineMechanical engineeringChemistryInternal medicineOptics

Abstract

fetched live from OpenAlex

• Synchrotron micro-CT enhanced visualization of internal cracks undetectable in 2D analysis. • Steel microstructure influenced hydrogen diffusion and trapping, affecting crack initiation and severity. • Simultaneous hydrogen ingress and stress resulted in more severe embrittlement. • Hydrogen retention, not just crack initiation, critically drives embrittlement and failure mode. Hydrogen embrittlement (HE) presents a major challenge to the integrity of steel pipelines, often leading to premature failure. Traditional methods using two-dimensional (2D) analysis of damaged structures, often overlook critical features related to failure. Hence, this study investigates the hydrogen embrittlement susceptibility of two pipeline steels, X60 and X65, using a combination of mechanical testing, hydrogen diffusion and trapping studies, microstructural characterization, and synchrotron micro-computed tomography (micro-CT) imaging. The results highlight the critical role of hydrogen trapping and retention in HE, with steel microstructure significantly affecting hydrogen uptake and diffusion as well as crack nucleation and propagation. Synchrotron micro-CT imaging provided more accurate crack pattern assessments than traditional 2D methods, revealing potential misinterpretations from 2D cross-sectional analysis. This study concludes that simultaneous hydrogen ingress and mechanical loading is more damaging than pre-charging with high hydrogen concentrations, and that hydrogen retention capacity plays a greater role in embrittlement behavior than crack initiation. The failure mechanism of the hydrogen-charged steels shifted from being plasticity-based to decohesion-driven, based on the hydrogen content and retention in the steel, which is in line with the unified HELP+HEDE model.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.229
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2025
Admission routes2
Has abstractyes

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