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Record W4407614982 · doi:10.1002/cjce.25645

Fines deposition during hydrotreating: Effects of catalyst size and bed arrangement

2025· article· en· W4407614982 on OpenAlexafffundvenue
Simon Kwao, V. Sundaramurthy, Ajay K. Dalai, John Adjaye

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2025
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsUniversity of Saskatchewan
FundersNatural Sciences and Engineering Research Council of CanadaSyncrude
KeywordsHydrodesulfurizationDeposition (geology)CatalysisCloggingRefining (metallurgy)Materials scienceEnvironmental scienceMetallurgyChemistryGeology

Abstract

fetched live from OpenAlex

Abstract Fines deposition presents a significant problem during the hydrotreating of bitumen‐derived gas oils. The accumulation of fines leads to reactor clogging and consequently, pressure drop buildup. At critical levels, the hydrotreating reactor must be prematurely shutdown, resulting in substantial economic losses for refineries. Hence, research into finding measures to address fines deposition is crucial and of interest to stakeholders in the refining industry. This research explored the effects of catalyst size and bed arrangement on fines deposition, with the goal of identifying strategies to obtain longer hydrotreating run times. Cold and hot flow fines deposition tests were conducted in three‐zone reactors using NiMo/γ‐Al 2 O 3 catalysts, with sizes ranging from 1.3 to 2.5 mm. Under cold flow conditions, maximum fines deposition was reached in 12, 14, and 25 days for 1.3, 1.6, and 2.5 mm catalyst sizes, respectively. For the hot flow tests, maximum fines deposition occurred in 15, 17, and 28 days for 1.3, 1.6, and 2.5 mm catalyst sizes, respectively. Thus, both flow tests suggested that reducing catalyst size accelerated fines deposition, primarily due to straining. However, when the catalyst bed was arranged with decreasing size from top to bottom of the reactor, the time to reach maximum fines deposition increased to 28 days (cold flow) and 34 days (hot flow). Therefore, configuring the catalyst bed to have a downward gradient of decreasing catalyst size is proposed as a potential strategy to extend hydrotreating run times.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.035
Threshold uncertainty score0.302

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.164
Teacher spread0.162 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2025
Admission routes3
Has abstractyes

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