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Influence of physicochemical conditions on liquid-liquid phase separation and stability of immunoglobulin Y for storage and application

2025· article· en· W4407848736 on OpenAlexaff
Yuzhang Hu, Mei Dang, Xiaoying Zhang

Bibliographic record

VenueInternational Journal of Biological Macromolecules · 2025
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicProtein purification and stability
Canadian institutionsUniversity of Guelph
Fundersnot available
KeywordsChemistryChromatographyLiquid liquidLiquid phaseSeparation (statistics)Chemical engineeringThermodynamicsComputer sciencePhysicsEngineering

Abstract

fetched live from OpenAlex

Liquid-liquid phase separation (LLPS) is a biological process and can lead to the formation of irreversible aggregates of functional proteins upon storage and administration, making it essential to predict and mitigate this phenomenon. Immunoglobulin Y (IgY), a unique class of antibody derived from egg yolk has broad applications in disease diagnosis, prophylaxis, and treatment. In this study, we observed the formation of droplet-shaped condensates of IgY under crowding conditions with polyethylene glycol 8000 (PEG 8000). To assess the relative contribution of different IgY domains to LLPS, we prepared the fragment antigen binding (Fab), fragment crystallizable (Fc) 3-4, and Escherichia coli-expressed IgY-Fc 2-4 domain. After PEG 8000 addition, the Fab fragments more propensity to aggregate, while Fc 3-4 and E. coli-expressed Fc underwent LLPS. Furthermore, we found that LLPS of IgY is influenced by electrostatic interactions. Recognizing the negative effects of LLPS on antibody efficacy, our study showed that the addition of arginine and lysine at low concentrations could prevent PEG-induced LLPS, enhancing IgY stability. These findings provide valuable insights into the optimization of IgY antibody applications and storage conditions, advancing our understanding of antibody stability in solution and facilitating the development of strategies to protect antibodies from aggregation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.257

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.341
Teacher spread0.328 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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