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Record W4408073075 · doi:10.1016/j.cej.2025.161105

Methane production and microbial adaptation in high-load vacuum-enhanced anaerobic digestion: Addressing ammonia and propionate toxicity

2025· article· en· W4408073075 on OpenAlexafffund
Ali Khadir, Basem Haroun, Eun-Kyung Jang, Domenico Santoro, John Walton, Ahmed Al‐Omari, Christopher Muller, Katherine Y. Bell, Wayne J. Parker, George Nakhla

Bibliographic record

VenueChemical Engineering Journal · 2025
Typearticle
Languageen
FieldEngineering
TopicAnaerobic Digestion and Biogas Production
Canadian institutionsUniversity of WaterlooWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPropionateAmmoniaAnaerobic digestionAnaerobic exerciseChemistryAmmonia productionAdaptation (eye)MethaneProduction (economics)Environmental chemistryMicrobiologyPulp and paper industryBiochemistryBiologyEngineeringOrganic chemistryPhysiology

Abstract

fetched live from OpenAlex

• IntensiCarb technology processed 6 times the OLR of conventional AD. • Methane yield decreased linearly with increasing propionate concentrations over 2.20 g/L. • Side-stream vacuum increased ammonia toxicity resilience by a factor of 3. • Population of propionate degraders in IC was different from conventional AD. • Methanosaeta dominated conventional AD, while Methanosarcinaceae dominated IC reactors. Ex-situ vacuum-enhanced anaerobic digestion (IntensiCarb-AD) of primary and thickened waste activated sludge (PS/TWAS) was tested at an organic loading rate (OLR) of 11.0–11.3 kg COD/m 3 -d. IC-AD reactors with similar solids retention times (SRT = 20 d) and OLR, were operated at hydraulic retention times (HRT) of 5 days (IF defined as SRT/HRT of 4) and 3.33 days (IF6). IF4 had a higher steady-state methane yield of 0.214 ± 0.009 L-CH 4 /gCOD fed compared to 0.148 ± 0.029 L-CH 4 /gCOD fed in IF6. COD removals of 53.5 %±2.25 % were obtained with IF4 but fluctuated with IF6 (37.0 %±7.25 %). Both IF4 and IF6 processed 6 times the OLR of a conventional AD with comparable volatile solids reduction efficiency. The relative instability in IF6 was linked to a greater reduction in microbial activity due to longer vacuum application and higher propionate concentrations (>2.20 g/L), which affected the performance of hydrogenotrophic methanogens. Methanosarcinaceae and Methanobacteriaceae populations were 10.8 % and 35.2 % more abundant in IF4 than in IF6, respectively, corroborating the significantly higher methane yields observed in IF4 compared with IF6. Ammonia recovery efficiencies of 52.0 % and 49.1 % were observed in IF4 and IF6 respectively. Batch ammonia toxicity tests indicated a higher inhibitory constant (K i ) for IC-AD (5.60–5.70 gN/L) compared to conventional AD (1.90 gN/L). Acetate degradation was effective even with ammonia and propionate concentrations as high as 2,000 mg/L and 4,000 mg/L, respectively.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.023
Threshold uncertainty score0.706

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.209
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2025
Admission routes2
Has abstractyes

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