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Effect of hydroxypropyl methylcellulose and ferric chloride on hypergolic ignition of solidified ethanol fuels

2025· article· en· W4408669192 on OpenAlexafffund
Jerin John, Purushothaman Nandagopalan, Ankur Miglani, Pranay Mudaliar, Seung Wook Baek

Bibliographic record

VenueCombustion and Flame · 2025
Typearticle
Languageen
FieldEngineering
TopicEnergetic Materials and Combustion
Canadian institutionsConcordia University
FundersNatural Sciences and Engineering Research Council of CanadaNational Research Foundation of Korea
KeywordsFerricChemistryEthanolIgnition systemChlorideMethanolInorganic chemistryNuclear chemistryOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

• Hypergolic ignition of reaction-driven solidified fuels with varying concentrations of hydroxylpropyl methylcellulose and ferric chloride has been investigated for the first time. • FTIR and TGA techniques has been used to study molecular interactions between hydroxylpropyl methylcellulose and ferric chloride. • Hypergolic ignition delay tests with 90 % H 2 O 2 reduced ignition delay with increase in the concentration of gellant and dopant. • Higher fuel temperature improved spreading and wetting behavior of H 2 O 2 droplets. • Solidification of ethanol using HPMC with FeCl 3 eliminates the need for a separate catalyst. This study investigates the hypergolic ignition of reaction-driven solidified ethanol (RDSE) fuels, focusing on the effects of varying concentrations of hydroxypropyl methylcellulose (HPMC) gellant and ferric chloride (FeCl 3 ) dopant. Fourier Transform Infrared Spectroscopy (FTIR) and thermogravimetric analysis (TGA) are employed to examine molecular interactions and thermal properties. FTIR results indicate that no new covalent bonds are formed upon adding FeCl 3 , whereas interactions primarily governed by weak hydrogen and ionic bonds. The apparent activation energy ( E a ) has been determined for the fuel samples using iso-conversional model-free kinetics approach and found that E a decreased with HPMC and FeCl 3 concentrations. Hypergolic ignition delay tests were attempted with the droplet study rocket grade hydrogen peroxide (90 % RGHP; H 2 O 2 ) as an oxidizer, demonstrated that increasing HPMC concentration by 3 wt.% reduced ignition delay by ∼20 %, while a 5 wt.% increase in FeCl 3 concentration led to a ∼25 % reduction. Higher fuel temperatures enhanced the wetting and spreading behavior of H 2 O 2 droplets, improving oxidizer-fuel interaction and reducing ignition delay. Overall, solidification of ethanol using HPMC with FeCl 3 eliminates the catalyst as FeCl 3 acts as both catalyst and binding agent.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.039
Threshold uncertainty score0.434

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.219
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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