MétaCan
Menu
Back to cohort
Record W4409195484 · doi:10.1016/j.elecom.2025.107919

Stability of silver/silver chloride quasi-reference electrodes under gamma radiation for corrosion measurements

2025· article· en· W4409195484 on OpenAlexafffund
Anqi Shi, Emmanuel Mena‐Morcillo, Taras Skotar, Reza Moshrefi, Mehran Behazin, Peter Keech, Samantha Michelle Gateman

Bibliographic record

VenueElectrochemistry Communications · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicAnalytical Chemistry and Sensors
Canadian institutionsNuclear Waste Management OrganizationWestern University
FundersNatural Sciences and Engineering Research Council of CanadaNuclear Waste Management Organization
KeywordsCorrosionElectrodeChlorideMaterials scienceRadiationSilver chlorideElectrochemistryInorganic chemistryChemistryAnalytical Chemistry (journal)MetallurgyOpticsPhysicsPhysical chemistryEnvironmental chemistry

Abstract

fetched live from OpenAlex

This study explored the long-term stability of silver/silver chloride (Ag/AgCl) quasi-reference electrodes (QREs) for in-situ electrochemical measurements under gamma radiation at room temperature. Compared to full half-cell REs, QREs enable low-volume experiments and avoid frit obstruction. Both ex-situ open circuit potential and in-situ internal reference probe measurements were employed to confirm the reliability of the Ag/AgCl QREs for at least 33 days. The electrodes were implemented successfully for in-situ electrochemical corrosion measurements of copper under radiation, important for nuclear waste storage applications. This work sets the standards for validating other (quasi) reference electrodes under harsh conditions and confirms the stability of AgCl coatings for implementation of QREs for small-scale radioelectrochemical experiments. • Ag/AgCl quasi-reference electrodes exhibit long-term stability under ionizing radiation. • Novel internal reference measurements validate their reliability for in-situ electrochemical analysis. • Ag/AgCl is a robust quasi-reference electrode material for monitoring copper corrosion in irradiated environments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.216
Threshold uncertainty score0.907

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.050
GPT teacher head0.302
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

Explore more

Same venueElectrochemistry CommunicationsSame topicAnalytical Chemistry and SensorsFrench-language works237,207