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Oxidative potential of ambient particulate matter from community sites in Alberta's oil sands region

2025· article· en· W4409412957 on OpenAlexafffundabout
Pourya Shahpoury, Jasmin K. Schuster, Tom Harner

Bibliographic record

VenueChemosphere · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsEnvironment and Climate Change CanadaTrent University
FundersEnvironment and Climate Change CanadaWood Buffalo Environmental AssociationTrent University
KeywordsParticulatesOil sandsEnvironmental scienceEnvironmental chemistryEnvironmental protectionEnvironmental engineeringWaste managementChemistryGeographyArchaeologyEngineeringAsphalt

Abstract

fetched live from OpenAlex

Air pollution is a major environmental health risk and it has been associated with various diseases and mortality worldwide. The inhalation of fine particulate matter (PM) is an important cause of health effects from air pollution with one of underlaying mechanisms involving the induction of oxidative stress in the body. Oil sands mining is a major economic sector and a notable source of air pollution in northern Alberta, Canada. Despite this, studies investigating the potential health impacts associated with exposure to air pollutants in the region are rare. For the first time in this work, using an acellular • OH assay, we studied the oxidative potential (OP) of fine (<2.5 μm diameter) and coarse (2.5–10 μm diameter) PM from four community sites in the vicinity of oil sands production facilities. OP OH was found to be dominated by fine PM, which on average accounted for 70 % reactivity of the studied PM size range. The highest OP OH was found at the most populated sites located south of the open pit mines and with mixed emission sources, suggesting a cumulative effect of oil sands and non-oil sands sources. Nevertheless, OP OH was relatively small compared to values reported for urban sites influenced by traffic and industrial emissions in Canada. OP OH variation could not be linked with a statistical significance to changes in the concentrations of PM, trace metals, and secondary inorganic salts but, for a small set of samples, OP OH was associated with organic carbon and potassium, which suggests the influence of reactive organic species from biomass combustion. A larger sample size will be needed in order to examine more closely the links between various OP metrics and the aerosol composition and sources in the region. This work provides a proof of concept to support future studies aimed at assessing potential health impacts associated with exposure to air pollutants in the oil sands region.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.240
Threshold uncertainty score0.484

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0020.002
Science and technology studies0.0020.000
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.224
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes3
Has abstractyes

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