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Record W4409485412 · doi:10.5006/c2023-18924

Influence of Alloying Elements on the Electrochemical Behavior of Cantor High Entropy Alloys in Chloride Solutions

2023· article· en· W4409485412 on OpenAlexaff
Emily Seto, Haoxiang Wang, Jing Liu

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEngineering
TopicHigh Entropy Alloys Studies
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsElectrochemistryChlorideHigh entropy alloysEntropy (arrow of time)Materials scienceThermodynamicsStatistical physicsMetallurgyChemistryPhysicsPhysical chemistryElectrodeMicrostructure

Abstract

fetched live from OpenAlex

Abstract FeCoCrNi-based high entropy alloys (HEAs) are often used as prototype model alloys and have been developed broadly through modifying or replacing constituents with other elements to serve in extremely harsh environments such as in nuclear and marine engineering. Most previous studies were focused on the microstructure, mechanical properties, and oxidation behavior of FeCoCrNi-based HEAs. To date, very little work has been published on the corrosion behavior of HEAs in aqueous environments. In this study, the corrosion behavior of Cantor HEAs, including Fe20Co20Cr20Ni20Cu20 (H4Cu20), Fe20Co20Cr20Ni-20Cu15Al5 (H4Cu15Al5), and Fe20Co20Cr20Ni20Cu10Al10 (H4Cu10Al10), also known as H4C alloys, are investigated in aerated 3.5 wt% NaCl solutions at room temperature via electrochemical measurements. A common stainless steel (UNS S30403), and the original Cantor HEA (Fe20Co20Cr20Ni20Mn20, H4Mn20) are also evaluated as comparisons. Results confirmed that the addition of Al into the FeCoCrNi-based HEA improves the general corrosion resistance of Cantor HEAs. Among all five alloys, H4Cu10Al10 has the best general corrosion resistance with the slowest cathodic kinetics. The main types of corrosion on these HEAs were interdendritic and pitting corrosion after anodic polarization. Polarization experiments and post-characterization revealed that although the H4C alloys exhibit low pitting potential and low resistance to pitting initiation, the formed localized corrosion was interdendritic corrosion rather than big pits. Overall, results indicate that there is no significant advantage of using Cantor HEAs over common stainless steel in terms of corrosion consideration in aqueous chloride environments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.120
Threshold uncertainty score0.430

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.231
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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