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Record W4409529595 · doi:10.1021/acs.analchem.4c05403

Interlaboratory Comparison Reveals State of the Art in Microplastic Detection and Quantification Methods

2025· article· en· W4409529595 on OpenAlexafffund
Dmitri Ciornii, Vasile‐Dan Hodoroaba, Nizar Benismail, Alina Maltseva, Jiamin Wang, Raquel Parra, Ronan Jézéquel, Justine Receveur, Dina Gabriel, Andreas Scheitler, Christa van Oversteeg, Jorg Roosma, Alex van Renesse van Duivenbode, Tim Bulters, Michela Zanella, Alessandro Paoletti Perini, Federico Benetti, Dóra Méhn, Georg Dierkes, Michael Soll, Takahisa Ishimura, Marius Bednarz, Guyu Peng, Lars Hildebrandt, Seung‐Kyu Kim, Jochen Türk, Felix Steinfeld, Jaehak Jung, Sang-Hee Hong, Eunju Kim, Hye-Weon Yu, Sven Klockmann, Christoph Krafft, Julia Süssmann, Shan Zou, Alexandra ter Halle, Andrea Mario Giovannozzi, Alessio Sacco, Mara Putzu, Dong-Hoon Im, Nontete Nhlapo, Priscilla Carrillo-Barragán, Natascha Schmidt, Dorte Herzke, Alessio Gomiero, Adrián Jaén-Gil, Damien Cabanes, Martin Doedt, Moritz Hawly, Huatao Mo, Justine Jacquin, Andy Mechlinski, Gbotemi A. Adediran, J.M. Andrade, Soledad Muniategui‐Lorenzo, Anja F. R. M. Ramsperger, Martin G. J. Löder, Christian Laforsch, Tanja Ćirković Veličković, Daniele Fabbri, Irene Coralli, Stefania Federici, Barbara M. Scholz‐Böttcher, Jacopo La Nasa, Greta Biale, Cassandra Rauert, Elvis D. Okoffo, Anna K. Undas, Lihui An, Volker Wachtendorf, Petra Fengler, Korinna Altmann

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMicroplastics and Plastic Pollution
Canadian institutionsNational Research Council Canada
FundersMinistry of Science and ICT, South KoreaKorea Institute of Marine Science and Technology promotionNational Institute of Fisheries ScienceHorizon 2020 Framework ProgrammeNorges ForskningsrådBundesministerium für Bildung und ForschungNational Natural Science Foundation of ChinaHelmholtz-GemeinschaftNational Research Foundation of KoreaNational Key Research and Development Program of ChinaNational Research Council CanadaNational Research FoundationMinistry of Oceans and FisheriesXunta de GaliciaGovernment of CanadaDeutsche ForschungsgemeinschaftHORIZON EUROPE Framework ProgrammeEuropean Partnership on MetrologyEuropean Commission
KeywordsChemistryEnvironmental chemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide In this study, we investigate the current accuracy of widely used microplastic (MP) detection methods through an interlaboratory comparison (ILC) involving ISO-approved techniques. The ILC was organized under the prestandardization platform of VAMAS (Versailles Project on Advanced Materials and Standards) and gathered a large number (84) of analytical laboratories across the globe. The aim of this ILC was (i) to test and to compare two thermo-analytical and three spectroscopical methods with respect to their suitability to identify and quantify microplastics in a water-soluble matrix and (ii) to test the suitability of the microplastic test materials to be used in ILCs. Two reference materials (RMs), polyethylene terephthalate (PET) and polyethylene (PE) as powders with rough size ranges between 10 and 200 μm, were used to press tablets for the ILC. The following parameters had to be assessed: polymer identity, mass fraction, particle number concentration, and particle size distribution. The reproducibility, S R, in thermo-analytical experiments ranged from 62%–117% (for PE) and 45.9%–62% (for PET). In spectroscopical experiments, the S R varied between 121% and 129% (for PE) and 64% and 70% (for PET). Tablet dissolution turned out to be a very challenging step and should be optimized. Based on the knowledge gained, development of guidance for improved tablet filtration is in progress. Further, in this study, we discuss the main sources of uncertainties that need to be considered and minimized for preparation of standardized protocols for future measurements with higher accuracy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.246
Threshold uncertainty score0.212

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.288
Teacher spread0.278 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations42
Published2025
Admission routes2
Has abstractyes

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