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Record W4409752819 · doi:10.1002/cjce.25712

Experimental methods in chemical engineering: Electron probe micro‐analysis— <scp>EPMA</scp>

2025· article· en· W4409752819 on OpenAlexaffvenue
Viviane de Oliveira Campos, Felipe Fernandes Barbosa, Ellen Kadja Lima de Morais, Dulce Maria de Araújo Melo, Jildimara de Jesus Santana, Gregory S. Patience

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2025
Typearticle
Languageen
FieldMaterials Science
TopicElectron and X-Ray Spectroscopy Techniques
Canadian institutionsPolytechnique Montréal
Fundersnot available
KeywordsElectron microprobeAnalytical Chemistry (journal)Materials scienceElectronChemistryMetallurgyPhysicsEnvironmental chemistryNuclear physics

Abstract

fetched live from OpenAlex

ABSTRACT Electron probe microanalysis (EPMA) is a non‐destructive spectroscopic technique to map the chemical composition—quantitative elemental distribution and layer thickness—with a micro‐scale resolution. An electron beam illuminates the surface of a sample and produces backscattered electrons (BSE), secondary electrons (SE), characteristic X‐rays, and light known as cathodoluminescence (CL). Combining energy dispersive spectrometry with wavelength‐dispersive spectrometry improves trace analysis and differentiates overlapping X‐ray lines, but the detection threshold is not much better than 100 ppm (parts per million). Implementing Monte Carlo simulation with better electronics and software are ongoing research areas to improve the method's precision, sensitivity, and spatial resolution. To detect Li, Be, and B ( 11) requires wavelength‐dispersive X‐ray spectroscopy (WDS), or soft X‐ray emission spectroscopy (SXES), or a combination of BSE/EDS method. Researchers in metallurgy & metallurgical engineering, mineralogy, geochemistry & geophysics, and mining & mineral processing apply the method most. Chemical engineering is ranked 21st among the 250 scientific categories that use the technique. It is also applied to reconstitute works of art and the antiquities. A bibliometric map identified four clusters of research and for each cluster the major nodes were: (1) geochemistry, (2) mechanical properties, microstructure, and alloys, (3) Fe, Cu, and Cr, and (4) phase equilibria.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.003
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.044
Threshold uncertainty score0.148

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0030.003
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0030.003
Science and technology studies0.0010.001
Scholarly communication0.0020.002
Open science0.0020.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0440.017

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.278
Teacher spread0.271 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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