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Record W4409834716 · doi:10.1021/acs.analchem.5c00079

A Rapid Testing Kit for 6PPD Screening in Rubber Products

2025· article· en· W4409834716 on OpenAlexafffund
Zhuoyuan Li, Lin-Na Xie, Pranav Nair, Kirsten Yeung, Oliver Meek, Juan Tao, Kyoshiro Hiki, Chunyan Hao, Hui Peng

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicEffects and risks of endocrine disrupting chemicals
Canadian institutionsMinistry of the Environment, Conservation and ParksAUG Signals (Canada)University of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaMinistère de l’Environnement, de la Protection de la nature et des ParcsOntario Ministry of Economic Development, Job Creation and Trade
KeywordsChemistryNatural rubberChromatographyOrganic chemistry

Abstract

fetched live from OpenAlex

N -(1,3-dimethylbutyl)- N′ -phenyl- p -phenylenediamine (6PPD) has received increasing attention due to its ubiquitous environmental occurrence and extreme aquatic toxicity of its oxidation product 6PPD-quinone. Given 6PPD’s application as an antioxidant in a wide array of rubber products, cost-effective detection of 6PPD is important for product and waste management. We herein developed a rapid testing kit for the detection (<10 min) of 6PPD in rubber products with low costs (<$1/sample), which was inspired by the observation of a red-colored product after 6PPD exposure to oxidants. The selectivity of this reaction was evaluated by 14 structurally diverse phenols and anilines. Interestingly, the protonated N -1,3-dimethyl butyl- N’ -phenyl quinone diimine (6QDI+H + ), rather than its neutral or radical counterparts, appeared to be the red-colored product with λ max = 490 nm. We further developed a “green” and user-friendly 6PPD rapid testing kit, which was further applied to a wide array of 50 rubber products. 6PPD was detected in 22 out of 50 samples, with a strong agreement ( R 2 = 0.896) observed between the results of the rapid testing kit and LC-MS. In summary, this study introduces a 6PPD rapid testing kit for users without requiring expertise in chemistry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.005
Threshold uncertainty score0.016

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0020.002
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0050.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.341
Teacher spread0.319 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes2
Has abstractyes

Explore more

Same venueAnalytical Chemistry→Same topicEffects and risks of endocrine disrupting chemicals→French-language works237,207→