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Record W4410493300 · doi:10.1371/journal.pone.0320584

Assessment of palladium concentration in drill cores using laser-induced breakdown spectroscopy (LIBS)

2025· article· en· W4410493300 on OpenAlexafffundabout
François Vidal, Samira Selmani, Ismail Elhamdaoui, Nessrine Mohamed, Paul Bouchard, Marc Constantin, Mohamad Sabsabi

Bibliographic record

VenuePLoS ONE · 2025
Typearticle
Languageen
FieldEngineering
TopicLaser-induced spectroscopy and plasma
Canadian institutionsNational Research Council CanadaUniversité LavalInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsLaser-induced breakdown spectroscopyPalladiumLaserRADIUSMaterials scienceSpectroscopyAnalytical Chemistry (journal)OpticsChemistryComputer scienceChromatographyPhysics

Abstract

fetched live from OpenAlex

Laser-induced breakdown spectroscopy (LIBS) appears to be a promising technique for rapid on-site assessment of precious metal concentrations in ores. However, a number of issues need to be considered for the optimal use of this technique in practical situations. This article focuses on the number of measurements (i.e., spectra or laser shots) required to assess the mean palladium concentration in drill cores from the Lac des Iles mine (Ontario, Canada). We have performed a probabilistic study of the accuracy of the mean palladium concentration obtained by LIBS as a function of the number of measurements at random locations. For this purpose, we first used the results of a detailed laser scan of the core surface and then a mathematical model of the probability density of the palladium distribution to explore the parameter space, in particular the effect of noise on the measurements. We show that for the 1-meter-long, 2-centimeter radius quarter core samples analyzed, a few thousand randomly sampled locations generally provide an assessment of the palladium concentration within useful confidence limits. For a typical laser repetition rate of 50 Hz, such an analysis is a matter of minutes compared to hours or days using conventional methods.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.027

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.265
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes3
Has abstractyes

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Same venuePLoS ONESame topicLaser-induced spectroscopy and plasmaFrench-language works237,207