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Record W4411085441 · doi:10.1021/acs.analchem.5c00076

Modular Centrifugal Microfluidics for Sample Preparation

2025· article· en· W4411085441 on OpenAlexaff
Ali Gholizadeh, Gabriel Mazzucchelli, Ana Amoroso, Tristan Gilet

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldEngineering
TopicMicrofluidic and Capillary Electrophoresis Applications
Canadian institutionsIONICS Mass Spectrometry (Canada)
FundersService Public de Wallonie
KeywordsChemistryMicrofluidicsModular designNanotechnologySample (material)Sample preparationChromatographyProgramming language

Abstract

fetched live from OpenAlex

Sample preparation is often a critical and labor-intensive step in molecular biology and analytical chemistry. It bottlenecks biological assays, where liquid-handling speed and technique influence the outcome. While automation improves efficiency, traditional systems such as robotic platforms remain costly, complex, and resource-intensive to manufacture. Centrifugal microfluidic devices provide liquid-handling operations at the microliter scale by using microfluidic channels and chambers engraved on disks (Lab-On-A-Disk, LOAD). However, their monolithic design limits flexibility and demands microfluidic expertise, thereby increasing prototyping time and costs, while discouraging broader adoption. To address these limitations, we introduce modular microfluidic chips that are integrable and functional on both LOAD platforms and commercial centrifuges, enabling broad laboratory use without additional equipment. These interchangeable modules perform specific functions─dispensing, metering, mixing, pooling, and collection─without requiring extra components for leak-proof interconnection. Their detachability from the rotating support allows fluid control through "flipping" relative to the centrifugal force. Additionally, they are compatible with multiwell plates and stackable in swinging-bucket centrifuges, enabling high-throughput sample preparation. As a proof of concept, an enzymatic assay was performed by using several assemblies of modules in parallel. After the reagents were mixed and transferred into a well plate, absorbance was measured at three antibiotic concentrations, confirming accurate volume control and reproducible measurements. This modular approach enhances miniaturization, compatibility, and affordability while reducing the reliance on expensive and bulky robotic systems. By simplifying workflows and improving flexibility, this provides an efficient alternative for rapid and scalable sample preparation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.006
Threshold uncertainty score0.019

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0060.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.239
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2025
Admission routes1
Has abstractyes

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