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Record W4411412363 · doi:10.1016/j.xcrp.2025.102659

Cryo-EM structures of artificial spider silk nanofibrils reveal insights into β sheet crystallization

2025· article· en· W4411412363 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueCell Reports Physical Science · 2025
Typearticle
Languageen
FieldMaterials Science
TopicSilk-based biomaterials and applications
Canadian institutionsnot available
FundersShanghai Institute of Organic Chemistry, Chinese Academy of SciencesChinese Academy of Sciences, Shanghai BranchScience and Technology Commission of Shanghai MunicipalityNational Natural Science Foundation of ChinaCanadian Anesthesiologists' SocietyChinese Academy of SciencesNational Science Foundation
KeywordsSpider silkSILKSpiderPolymer scienceCrystallizationMaterials scienceBiologyEngineeringChemical engineeringComposite materialZoology

Abstract

fetched live from OpenAlex

Spider silk is renowned for its exceptional mechanical properties, including its strength, toughness, and lightweight nature, making it a promising biomaterial. These properties largely arise from β sheet crystalline regions composed of poly(A) sequences, formed via liquid-liquid phase separation (LLPS). However, its nanoscale dimensions and disordered segments complicate structural characterization. In this study, we investigate an artificial spider silk protein, replacing poly(A) motifs with amyloidogenic peptides (GDVIEV) that promote β sheet formation. This replacement facilitates LLPS and the formation of nanofibrils with periodic structures resembling the β sheet conformation of natural spider silk. Using cryoelectron microscopy, we identify three different fibril polymorphs. The GDVIEV peptides predominantly adopt β sheet structures in the nanofibril core, stabilized by hydrogen bonds and hydrophobic interactions. These findings enhance our understanding of the self-assembly mechanisms and structural organization of spider silk, providing valuable insights for the development of biomimetic silk materials and the design of artificial proteins.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.040
Threshold uncertainty score0.548

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.268
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it