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Record W4411466269 · doi:10.1002/adem.202500503

Incorporation of Fe<sub>2</sub>O<sub>3</sub> Spacer Molecules in Microwave‐Exfoliated Graphene Oxide as Efficient Electrodes for Simultaneous Detection of Cd<sup>2+</sup>, Pb<sup>2+</sup>, and Hg<sup>2+</sup> in Water

2025· article· en· W4411466269 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAdvanced Engineering Materials · 2025
Typearticle
Languageen
FieldChemistry
TopicElectrochemical Analysis and Applications
Canadian institutionsUniversity of Waterloo
FundersKarpagam Academy of Higher Education
KeywordsGrapheneOxideMaterials scienceMetal ions in aqueous solutionNanomaterialsElectrodeElectrochemistryIonMoleculeNanoparticleMetalNanotechnologyAnalytical Chemistry (journal)Inorganic chemistryChemistryPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Toxic adverse effects to human beings caused by heavy metal ions resemble a serious threat to mankind and often appear in the journal headlines. However, simultaneous detection of heavy metal ions using analytical tools is challenging. In this regard, simultaneous electrochemical detection of Cd 2+ , Pb 2+ , and Hg 2+ ions in water is presented using iron oxide (Fe 2 O 3 ) nanostructures as spacers incorporated between microwave‐exfoliated graphene oxide (MEGO). First, Fe 2 O 3 nanostructures are synthesized using ferric nitrate in presence of poly(vinylpyrrolidone) and followed by their in‐situ incorporation into expanded graphene oxide (GO). Exfoliated GO accommodates large amount of Fe 2 O 3 nanoparticles via microwave‐assisted method, minimizing the restacking of GO sheets. Consequently, Fe 2 O 3 ‐incorporated MEGO (Fe 2 O 3 ‐MEGO) fabricated on screen‐printed electrodes (SPE) demonstrate well‐separated anodic peak potentials at −0.65, −0.45, and +0.27 V for Cd 2+ , Pb 2+ , and Hg 2+ ions. Moreover, Fe 2 O 3 ‐MEGO/SPE electrode exhibits wide linear range (0.4 to 74.78 μM), high sensitivities (8.11, 9.59, and 3.01 μA μM −1 cm −2 ) with low detection limits (0.2, 0.17, and 0.25 μM) for Cd 2+ , Pb 2+ , and Hg 2+ ions, respectively. Therefore, this kind of incorporating nanomaterials as spacer molecules between GO allows for the design of alternative pathways to minimize restacking of GO and to increase sensitivity toward multiple targeted species.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.306
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.196
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it