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Record W4411548143 · doi:10.1002/cjce.70006

Study on the coupling effect of salt concentration on hydrate formation kinetics under different water saturation levels

2025· article· en· W4411548143 on OpenAlexvenueno aff
Xiangchun Jiang, Guiyang Ma, Siyu Liu, Ping Wang, Hao Wang, Xiao Wang

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMethane Hydrates and Related Phenomena
Canadian institutionsnot available
Fundersnot available
KeywordsKineticsSaturation (graph theory)HydrateSalt (chemistry)Coupling (piping)ChemistryWater saturationMaterials scienceChemical engineeringPhysical chemistryMathematicsPhysicsPorosityComposite materialOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Abstract The formation of hydrates provides a safe and efficient solution for the storage, transportation, and distribution of natural gas. The rapid generation of natural gas hydrates is one of the current research orientations. This paper focuses on studying the effects of different water saturations and salt concentrations on the generation kinetics and morphology of methane hydrates in complex systems, and fully considers the changes in the randomness characteristics of hydrate nucleation caused by these two factors. The experimental results show that with the increase of water saturation, the induction time of hydrate formation first decreases and then increases, while the randomness of the induction period gradually decreases and the distribution becomes more concentrated. Among them, a water saturation of 70% is relatively favourable for the formation of hydrates, with a shorter and more concentrated induction period. In addition, the magnitude of the salt concentration can affect the nucleation of hydrates. As the salt concentration increases, its effect on hydrate nucleation changes from promotion to inhibition. Therefore, there exists an optimal salt concentration range for promoting hydrate nucleation, but this optimal promotion range is different in systems with different water saturations. At a water saturation of 70%, the promotion range of the salt concentration on hydrate nucleation is larger. Therefore, water saturation and salt concentration have a coupling effect on the formation of hydrates. This study explains the reasons for the inconsistent effects of salt concentration on hydrate formation at present, and provides unique insights into the mechanism of hydrate formation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.203
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical Engineering→Same topicMethane Hydrates and Related Phenomena→French-language works237,207→