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Record W4412632503 · doi:10.1021/acsestair.5c00100

Oil Sands Facilities Are an Emission Source of Naphthenic Acid Fractional Compounds to the Atmosphere

2025· article· en· W4412632503 on OpenAlexafffundabout
Samar G. Moussa, John Liggio, Jeremy J. B. Wentzell, Ralf M. Staebler, Zoey Friel-Bartlett, Meguel Yousif, Yuan You, Andrea Darlington, Katherine Hayden, Shao‐Meng Li

Bibliographic record

VenueACS ES&T Air · 2025
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsEnvironment and Climate Change Canada
FundersEnvironment and Climate Change Canada
KeywordsNaphthenic acidOil sandsAtmosphere (unit)Environmental sciencePetroleum engineeringChemistryWaste managementGeologyMaterials scienceEngineeringOrganic chemistryAsphaltPhysicsMeteorologyComposite material

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide The oil sands (OS) region in Canada hosts one of the world’s largest unconventional crude oil deposits in the form of bitumen, which, when extracted, generates substantial tailings/wastewater that are stored in on-site ponds. Naphthenic acid fractional compounds (NAFCs), a complex mixture of alkyl-substituted acyclic and cycloaliphatic organic acids, are natural bitumen components known for their ecological toxicity and are concentrated during the extraction process into tailings ponds, where they are assumed to remain confined to the aqueous phase. Here, we quantify the emissions of up to 275 NAFCs to the atmosphere from a tailings pond and from facility-wide operations at major OS facilities. The results indicate that, despite the absence of NAFC air emissions in inventories, large quantities are emitted to the atmosphere, likely originating from surface photochemical and/or biodegradation processes. Emission rates across entire operations ranged from 3509 to 7286 kg h –1, translating to annual emissions of 1163–2660 tonnes from both primary and secondary sources. The findings imply that NAFC air emissions may serve as a key pathway for these chemicals to enter the environment, potentially impacting downwind ecosystems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.744
Threshold uncertainty score0.435

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.246
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes3
Has abstractyes

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