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Record W4412728992 · doi:10.1021/acsomega.5c03051

Physical Chemistry of Irregular Mixtures: A Chemical Kinetics Scan over the Collection of Montmorillonite Sorption Sites

2025· article· en· W4412728992 on OpenAlexafffund
Donald S. Gamble

Bibliographic record

VenueACS Omega · 2025
Typearticle
Languageen
FieldPhysics and Astronomy
TopicSpectroscopy and Quantum Chemical Studies
Canadian institutionsSaint Mary's University
FundersSaint Mary’s University
KeywordsSorptionMontmorilloniteKineticsChemistryChemical engineeringChromatographyEnvironmental chemistryOrganic chemistryAdsorptionEngineeringPhysics

Abstract

fetched live from OpenAlex

The simultaneous protection of food crops, soil, and water has been an ongoing issue for over 70 years. The technology required for the control of this has been stalled by one key fact. Soil is the ultimate example of physically and chemically irregular mixtures. Soils are also dynamic. Even soil components are irregular mixtures. The voluminous accumulation of related publications is all based on the assumption that the application of the correct physical chemistry is impossible for such mixtures. The research objective reported here is the demonstration that the correct chemical kinetics can be applied to an irregular mixture. The irregular mixture of montmorillonite sorption sites for atrazine is an example. Montmorillonite is one of the many crystalline aluminosilicates found in the Earth's crust. Weathering will add crystal lattice defects in addition to those predicted by the second law of thermodynamics. An irregular mixture of sorption sites for an organic compound was expected. An irregular mixture can be quantitatively characterized by an experimental scan of its components. An atrazine solution was used for two types of scans. A law of mass action scan over the reaction time revealed one set of sorption sites in which sorption equilibrium was established. This was not found for other sorption sites. Second-order chemical kinetics for sorption yielded the kinetic rate coefficients that characterize nonlinear kinetics. The scans of the kinetic rate coefficients over the numbers of filled sorption sites resolved the mixture of sorption sites into separate sets. These scan methods should be applied to environmentally important cases of contaminated agricultural soils.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.349

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.247
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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