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Record W4412848686 · doi:10.1021/acs.est.5c03754

Exploring the Long-Term Human Exposure to Short-, Medium-, and Long-Chain Chlorinated Paraffins under Variant Environmental Release Trends and Patterns

2025· article· en· W4412848686 on OpenAlexafffundabout
Chengkang Chen, Li Li, Frank Wania

Bibliographic record

VenueEnvironmental Science & Technology · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsThe Scarborough HospitalUniversity of Toronto
FundersNational Institute of Environmental Health SciencesNatural Sciences and Engineering Research Council of Canada
KeywordsEnvironmental science

Abstract

fetched live from OpenAlex

Releases of chlorinated paraffins (CPs) have led to long-term human exposure globally. Differences in CP use patterns (indoors vs outdoors) and temporal release trends in different regions may be reflected in differences in the extent and pathways of long-term exposure to CPs between human populations. We used the dynamic mechanistic model PROTEX to simulate releases and environmental fates of CPs in China, Canada, and Europe from 1930 to 2020 and contrast the resultant exposures for different birth cohorts. Predicted environmental and human body concentrations agree with measurements from the three regions. Far-field exposure pathways dominate for all cohorts even in China where CP indoor use is high. Longitudinal exposure trends differ between generations and regions due to the divergent release trends. Perinatal exposure causes high body concentrations in infants and children born in years with peak releases. Due to human elimination half-lives that are short relative to the period of release, cross-sectional concentration-age trends have similar shapes regardless of release trend and sampling time. These results imply that whereas use patterns and release trends add to the influence of physicochemical properties on relative exposure pathway importance and cross-sectional concentration-age trends, the release trends are the main factors shaping longitudinal exposure trends.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.060
Threshold uncertainty score0.119

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.242
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes3
Has abstractyes

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Same venueEnvironmental Science & Technology→Same topicToxic Organic Pollutants Impact→French-language works237,207→