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Record W4412930816 · doi:10.1016/j.clay.2025.107950

Reactivity assessment of calcined illite, kaolinite, and montmorillonite in R3 mixtures

2025· article· en· W4412930816 on OpenAlexafffund
Pengfei Zhao, Karl Peterson

Bibliographic record

VenueApplied Clay Science · 2025
Typearticle
Languageen
FieldEngineering
TopicConcrete and Cement Materials Research
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsMontmorilloniteIlliteKaoliniteClay mineralsCalcinationReactivity (psychology)GeochemistryGeologyMineralogyChemistryOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

This study evaluates the pozzolanic reactivity of calcined illite, kaolinite, and montmorillonite using the more recently standardized rapid, relevant, and reliable (R 3 ) test methods as specified in ASTM C1897. The reactions involving calcite and the calcined clay minerals were examined by comparing the cumulative heat release in the R 3 mixtures with and without calcite, and by analyzing the hydrated R 3 mixtures using X-ray diffraction (XRD), thermogravimetric analysis (TGA), and scanning electron microscopy (SEM). The results indicate that the R 3 reactivity of calcined clay minerals exhibits a positive linear relationship with the number of hydroxyl groups present in their original mineral structures. Strong correlations were observed among cumulative heat release, bound water content, and dehydroxylation mass loss of clay minerals. This suggests that the dehydroxylation mass loss can be used as an indicator for the initial screening of potential clay sources for use as supplementary cementitious materials (SCMs). However, the optimal calcination temperatures for illite and montmorillonite do not fall within their dehydroxylation temperature ranges. While calcite has a limited impact on the cumulative heat release, it facilitates the formation of monocarbonate (C 4 A C ¯ H 11 ) and enhances its uniform distribution in the calcined kaolinite R 3 mixture. In comparison, the reactions involving calcite with calcined illite and montmorillonite in their R 3 mixtures are limited.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.300
Teacher spread0.290 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2025
Admission routes2
Has abstractyes

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