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Record W4413758184 · doi:10.1016/j.xinn.2025.101089

Hydrogen crossover raises serious concerns on proton exchange membrane water electrolyzer

2025· article· en· W4413758184 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Innovation · 2025
Typearticle
Languageen
FieldEnergy
TopicHybrid Renewable Energy Systems
Canadian institutionsUniversity of Calgary
FundersNational Key Research and Development Program of ChinaKey Technologies Research and Development ProgramChongqing Postdoctoral Science Special FoundationNational Natural Science Foundation of China
KeywordsCrossoverProton exchange membrane fuel cellElectrolysisHydrogenElectrolysis of waterProtonEnvironmental scienceMembraneMaterials scienceChemistryComputer sciencePhysicsNuclear physicsElectrodeElectrolyte

Abstract

fetched live from OpenAlex

Green hydrogen plays a crucial role in the modern energy system, especially considering its production with the input of renewable electricity. Proton exchange membrane water electrolysis is favored for producing green hydrogen with renewable electricity, because of its high efficiency, rapid start-up, and quick adaptation to electricity changes. However, the hydrogen crossover issue gradually attracts significant attention under variable electricity input. The hydrogen crossover mechanism is proposed, with emphasis on its aggravation during the frequent start-stop cycles. The preliminary experimental observations and theoretical insights are reported to assess the hydrogen crossover rate under constant and dynamic operating conditions. Dynamic operation can particularly intensify the hydrogen permeation, increasing anode-side hydrogen volume fraction in oxygen and membrane degradation, thereby aggravating the safety risk and reducing efficiency. Several possible mitigation strategies, such as catalytic layer design, membrane material optimization, and operational condition control, are proposed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.356
Threshold uncertainty score0.493

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.267
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it