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Record W4414113045 · doi:10.1021/acsapm.5c02895

Hydrophobic, Mechanically Robust, and UV-Blocking Paper Enabled by Lignin Reinforcement

2025· article· en· W4414113045 on OpenAlexaff
Qiang Wang, Jinshan Zhang, Xin Li, Xiujing Liu, Shanshan Liu, Yingchao Wang, Pedram Fatehi

Bibliographic record

VenueACS Applied Polymer Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced Cellulose Research Studies
Canadian institutionsLakehead University
FundersTaishan Scholar Project of Shandong ProvinceNatural Science Foundation of Shandong ProvinceNational Natural Science Foundation of China
KeywordsLigninHardwoodCelluloseSoftwoodAbsorption of waterUltimate tensile strengthCellulose fiber

Abstract

fetched live from OpenAlex

Traditional paper is sensitive to water due to the strong capillary action and abundance of hydrophilic hydroxyl groups in cellulose. Inspired by outstanding properties of lignin, i.e., hydrophobicity, UV-blocking, and thermal stability, lignin-filled hardwood paper (LHP) was produced for various advanced applications. To enhance the lignin retention on the cellulose fibers, we mechanically beat the fibers to different degrees. Results showed that intensive beating made the fibers more fibrous, which significantly increased the lignin retention on the fibers. Benefiting from these changes, more lignin interacted with cellulose fibers, resulting in an increase in the hydrophobicity of lignin-filled hardwood paper (water contact angle (WCA) increased from 42 to 109°). Meanwhile, the water vapor transmission rate (WVTR) of LHP-90 °SR was only half that of the control (786 g/m 2 ·24 h), and its water absorption was as low as 49%. These data further confirmed the excellent hydrophobic properties of LHP-90 °SR, which was attributed to the phenylpropane units and aromatic groups in the lignin molecules. Due to the dense fiber network formed by intensive beating, the interaction between lignin and cellulose was strengthened by hydrogen bonding, thus leading to a remarkable improvement in the tensile strength of lignin-filled hardwood paper from 1 to 41.36 MPa. In addition, lignin filling not only made LHP-90 °SR effective in shielding UV rays but also endowed it with good thermal stability. This research revealed a viable approach to manufacture hydrophobic, thermostable, and UV-blocking paper with high strength for advanced food packaging applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.247
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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