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Record W4414213446 · doi:10.3390/liquids5030023

Bifunctional HLD–NAC for Clove Oil Microemulsions

2025· article· en· W4414213446 on OpenAlexafffund
Jiaxin Tan, Edgar Acosta

Bibliographic record

VenueLiquids · 2025
Typearticle
Languageen
FieldChemistry
TopicSurfactants and Colloidal Systems
Canadian institutionsUniversity of Toronto
FundersMitacs
KeywordsMicroemulsionBifunctionalHeptanePulmonary surfactantPhase (matter)EugenolLecithinDistillation

Abstract

fetched live from OpenAlex

Clove oil is an essential oil used in food and pharmaceutical applications, with a market value of 300+ million dollars per year. Microemulsions have been used as effective clove oil delivery vehicles and could also be used to develop new extraction processes from clove buds. Eugenol, the main component of clove oil, is a polar oil that behaves as a surfactant and as an oil. This bifunctional behavior makes formulating clove oil microemulsions a challenging task. Here, we used a version of the Hydrophilic–Lipophilic Difference (HLD) + Net-Average Curvature (NAC) model that incorporates the bifunctional polar oil model to predict and fit the phase behavior of lecithin (surfactant) + polyglycerol-10 caprylate (hydrophilic linker) microemulsions using mixtures of heptane and clove oil as the oil phase. Using HLD-NAC parameters from the literature, the predicted HLD-NAC curves reproduced the expected phase transitions and the trends in Eugenol segregation toward the surfactant layer. Using these literature parameters as an initial guess to fit the experimental phase volumes produced accurate calculated phase volumes, and predicted interfacial tensions. This work demonstrates the application of heuristics and databases of HLD-NAC parameters in predicting the complex phase behavior of surfactant–oil–water (SOW) systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.255
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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