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Record W4414555997 · doi:10.1021/acs.est.5c06941

Photodegradation Driven by Visible Light Exceeds Biodegradation across a Range of Environmental Conditions during the Initial Hours after an Oil Spill

2025· article· en· W4414555997 on OpenAlexafffund
Alice C. Ortmann, Brian Robinson, Ho-Yin Poon, Thomas King

Bibliographic record

VenueEnvironmental Science & Technology · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMicrobial bioremediation and biosurfactants
Canadian institutionsBedford Institute of Oceanography
FundersFisheries and Oceans CanadaGovernment of Canada
KeywordsPhotodegradationAbiotic componentBiodegradationOil spillDegradation (telecommunications)Aquatic ecosystemPollutantMicrobial biodegradation

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Degradation of oil compounds, mediated by microbes or abiotic factors, after a spill into aquatic environments is important for ecosystem recovery; however, factors controlling these processes in natural waters remain poorly characterized. Six experiments representing a range of environmental conditions measured the loss of n -alkanes and polycyclic aromatic compounds (PACs) from a crude oil over 72 h due to biodegradation and abiotic processes when exposed to visible light. On average, 22.8% (±12.6) of n -alkanes and 32.7% (±14.0) of PACs were removed in the live incubations compared to 19.1% (±19.3) of n -alkanes and 31.7% (±12.3) of PACs when microbial activity was inhibited by the addition of mercuric chloride. Substantial biodegradation was only observed in the warm, freshwater incubation. Additional experiments determined that most of the abiotic degradation could be attributed to photodegradation mediated by visible light. No clear link was observed between the environmental conditions and abiotic losses of oil compounds, indicating complex interactions between light, photosensitizers, and organisms. These experiments demonstrate that a significant proportion of the n -alkanes and PACs may be removed from a surface oil spill through photodegradation mediated by both visible and UV light, along with biodegradation, within a few days.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.235
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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