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Record W4414750921 · doi:10.1021/acs.analchem.5c04254

State of Charge in a Vanadium Redox Flow Battery Measured via <sup>1</sup>H MR Relaxation with Low Field Portable Magnets

2025· article· en· W4414750921 on OpenAlexafffund
Andrés Ramírez Aguilera, Florea Marica, C. Adam Dyker, Bruce J. Balcom

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsUniversity of New Brunswick
FundersNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsVanadiumFlow batteryState of chargeBattery (electricity)ElectrolyteRelaxation (psychology)MagnetAnodeCathode

Abstract

fetched live from OpenAlex

Vanadium redox flow batteries offer a promising solution for medium- to large-scale energy storage applications. Accurately monitoring the state of charge (SOC) of these batteries is crucial for optimizing long-term performance and ensuring effective battery control. Electrolyte crossover and side reactions can degrade battery performance, but traditional electrochemical techniques are often inadequate for diagnosing these issues. This study introduces a novel 1 H magnetic resonance approach to estimate the SOC by analyzing the bulk relaxation times, T 1 and T 2, in the electrolyte. The basis of the measurement is the paramagnetic relaxation enhancement effect of vanadium ions on the bulk solution. The four different vanadium oxidation states in the redox flow battery have very different effects on the bulk relaxation times. The different relaxivities of these four species permit the determination of concentration. The measurement employs two MR devices, one measuring the cathode electrolyte and one measuring the anode electrolyte. The magnets are small inexpensive, permanent magnets, Proteus magnets, with a 1 H resonance frequency of 20 MHz. To the best of our knowledge, this is the first analytical MR measurement employing two discrete MR magnets in close proximity. The prospect exists for simultaneous measurement with the two MR devices, although measurements are sequential in this study. We demonstrate how 2D maps correlating T 1 with T 1, T 2 with T 2, and T 1 with T 2, measured from both sides of the battery, can effectively “map” the SOC during operation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.156
Threshold uncertainty score0.691

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.227
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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