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Record W4415939363 · doi:10.1016/j.envres.2025.123282

Methylmercury bioaccumulation and biomagnification in streams within forested catchments defoliated by spruce budworm

2025· article· en· W4415939363 on OpenAlexafffundabout
Kadiri Ju, Karen A. Kidd, Carl P. J. Mitchell, Erik J. S. Emilson

Bibliographic record

VenueEnvironmental Research · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMercury impact and mitigation studies
Canadian institutionsCanadian Forest ServiceThe Scarborough HospitalNatural Resources CanadaUniversity of TorontoMcMaster University
FundersNatural Resources CanadaForest Protection LimitedJarislowsky FoundationCanada Foundation for InnovationNatural Sciences and Engineering Research Council of CanadaMinistère des Forêts, de la Faune et des Parcs
KeywordsMethylmercurySpruce budwormBioaccumulationBiotaTroutTrophic levelBiomagnificationWater qualityFood webWatershed

Abstract

fetched live from OpenAlex

Though outbreaks of defoliating insects are a widespread, natural disturbance in Canadian boreal forests and their magnitude and duration are increasing in recent years, we have little understanding of the impacts on stream ecosystems. Herein we examined the fate of mercury (Hg), a toxic element affected by other landscape-scale forest disturbances, in twelve stream food webs in Gaspé Peninsula, Québec, Canada, that ranged in their severity of watershed defoliation from spruce budworm ( Choristoneura fumiferana ). Basal food sources (coarse and fine particulate organic matter, and biofilms), several macroinvertebrate taxa, and fish (brook trout [ Salvelinus fontinalis ] and slimy sculpin [ Cottus cognatus ]) were sampled in 2019 and 2020 and analyzed for stable isotopes of C and N, methylmercury (MeHg) or total Hg (THg, fish only). Hierarchical partitioning models were used to identify relative importance among landscape and local water quality variables, and they explained 76 and 65% of variation in brook trout THg and carnivorous invertebrate (Chloroperlidae, Rhyacophila , Parapsyche ) MeHg levels, respectively, with dissolved organic carbon (DOC) as the main driver increasing biotic mercury levels. Trophic magnification slopes (TMS) (calculated as log 10 Hg vs. δ 15 N) ranged from 0.27-0.38 across all watersheds but were not related to defoliation severity or DOC concentrations. Collectively, these findings suggest that local measures of water quality are more important drivers of Hg bioaccumulation in stream biota than landscape disturbances caused by forest defoliation by spruce budworm.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.787
Threshold uncertainty score0.428

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.039
GPT teacher head0.360
Teacher spread0.321 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes3
Has abstractyes

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