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Record W4417190595 · doi:10.1111/gwmr.70028

Facilitated Transport of Organic Contaminants in a High Concentration, Multicomponent Plume

2025· article· en· W4417190595 on OpenAlexfundno aff
D. M. Mackay, B. Myller, Gino C. Bianchi‐Mosquera, Bruce D. Honeyman, Michael Schirmer, R. M. Allen‐King, William P. Ball, Robert L. Stollar

Bibliographic record

VenueGroundwater Monitoring & Remediation · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicGroundwater flow and contamination studies
Canadian institutionsnot available
FundersU.S. ArmyU.S. Geological SurveyUniversity of WaterlooJohns Hopkins UniversityColorado Department of Public Health and Environment
KeywordsPlumeSorptionContaminationAquiferPollutionWater pollutionOrganic chemicalsHazardous wastePanache

Abstract

fetched live from OpenAlex

Abstract A field experiment evaluated the transport of organic contaminants in a plume from hazardous waste disposal areas at the Rocky Mountain Arsenal. The plume contained many xenobiotic contaminants, with widely varying expected mobilities. In laboratory tests, the aquifer sediments had shown significant capacity for sorption of organic contaminants from synthetic groundwater, suggesting contaminants’ mobilities in situ could have been retarded. Sediment cores showed sorbed concentrations of contaminants at or below detection levels, suggesting sorption in situ was minimal. The field experiment made direct observations of organic contaminant transport under plume conditions by flushing tracer‐amended organic‐free water through the plume. No contaminants were retarded in their migration compared to the tracer, suggesting negligible sorption of the contaminants in situ. The concentration of colloids, cosolvents (such as alcohols and ketones), and anionic surfactants in the plume were too low to have had a significant effect on contaminant migration. Non‐ionic surfactants, though not monitored, could have reduced sorption somewhat if they had constituted a significant fraction of the uncharacterized dissolved organic carbon. Micro‐ or nano‐plastic particles, though monitored only indirectly, are deemed unlikely to have significantly affected organic solute transport. Microemulsions may have been present and facilitated the transport of contaminants, but only indirect evidence was obtained. Although the specific reasons for the enhanced mobility of organic contaminants could not be confirmed, this research is the first to show that unknown plume components can be responsible for the suppression of sorption, suggesting new lab research is needed to expand understanding of factors affecting sorption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.046
Threshold uncertainty score0.590

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.224
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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