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Record W6921861281 · doi:10.1021/jp303780m.s001

Group Additivity Values\nfor Estimating\nthe Enthalpy of Formation of Organic Compounds: An Update and Reappraisal.\n2. C, H, N, O, S, and Halogens

2016· article· en· W6921861281 on OpenAlexaff

Bibliographic record

VenueFigshare · 2016
Typearticle
Languageen
FieldChemistry
TopicChemical Thermodynamics and Molecular Structure
Canadian institutionsUniversity of Ottawa
Fundersnot available
KeywordsAdditive functionHalogenGroup (periodic table)BenzeneEnthalpyPyridineVariety (cybernetics)

Abstract

fetched live from OpenAlex

This study extends a previous publication on group additivity\nvalues\n(GAVs) for the elements C, H, and O, to include the elements nitrogen,\nsulfur, and the halogens. The present state and utility of the Benson\nadditivity schemes for estimating the enthalpy of formation (Δ<sub>f</sub><i>H</i><sup>0</sup>) of organic compounds are again\ndescribed, extending them to include more elements. Old and new GAVs\nfor a wide variety of compounds are provided and are revised where\nnecessary. When new terms are proposed, or old ones are significantly\naltered, the rationale for so doing is presented. GAV derived ring\nstrain values for benzene and pyridine indicate that the aromatic\nstabilization of each is essentially the same. As before, the thermochemical\nconsequences of replacing one functional group by another are also\nshown, thus permitting quick shortcuts to the estimation of new Δ<sub>f</sub><i>H</i><sup>0</sup> values.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.126
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0080.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.235
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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