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Record W6939456852 · doi:10.6084/m9.figshare.22612933

Additional file 6 of Determinants of substrate specificity in a catalytically diverse family of acyl-ACP thioesterases from plants

2023· article· en· W6939456852 on OpenAlexaff

Bibliographic record

VenueFigshare · 2023
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicBiochemical Acid Research Studies
Canadian institutionsCarleton University
Fundersnot available
KeywordsMass spectrumFatty acidDerivative (finance)Mass spectrometrySubstrate (aquarium)Spectral line

Abstract

fetched live from OpenAlex

Additional file 6: Fig. S3. EI mass spectra of compounds detected in media from K27(DE3) E. coli cultures expressing ALTs. β-keto fatty acids secreted into culture media were chemically decarboxylated to methylketones prior to GC-MS analysis. Standard spectra used for compound identification are shown to the right of sample spectra. Fully reduced free fatty acids and saturated methylketones were identified by comparison to standard spectra from the NIST 17 Mass Spectral Library. Monounsaturated methylketones were identified by comparison to spectra previously obtained by Goh et al. [30]. 3-hydroxy fatty acids were identified based on the presence of their trimethylsilyl (TMS) derivatives in silylated samples. Mass spectra of the 2TMS derivatives of 3-hydroxy fatty acids were compared to standard spectra in the NIST 17 library, with the exception of 7(Z)-3-hydroxyhexadec-7-enoic acid, which is unlisted. The 2TMS derivative of 7(Z)-3-hydroxyhexadec-7-enoic acid was identified based the presence of the molecular ion (m/z = 386) and prominent ion fragments characteristic of both the 2TMS derivative of a 3-hydroxy fatty acid (m/z = 73, m/z = 147, m/z = 233, M+ − 31) and the TMS derivative of a monounsaturated fatty acid (M+ − 169, M+ − 90). Indole, a quorum sensing molecule, was present in media from all induced cultures.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Dataset · Consensus signal: Dataset
Teacher disagreement score0.866
Threshold uncertainty score0.678

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.3220.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.052
GPT teacher head0.285
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreDataset

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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