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Record W6958509328 · doi:10.6084/m9.figshare.13675627

Development of a sustainable ternary magnetic nanocomposite GCNI for efficient and synergistic photodegradation of Rhodamine B under solar irradiation: kinetic and mechanistic studies

2021· article· en· W6958509328 on OpenAlexaff

Bibliographic record

VenueFigshare · 2021
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsUniversity of ManitobaCancerCare Manitoba
Fundersnot available
KeywordsRhodamine BPhotodegradationTernary operationNanocompositeAdsorptionDegradation (telecommunications)Magnetic separationKineticsMagnetic nanoparticles

Abstract

fetched live from OpenAlex

In this study, a novel sunlight-active ternary magnetic nano-photocatalyst GCNI (Nanozero valent Iron @ Graphene oxide and Chitosan support) was fabricated. This easily retrievable magnetic nanocomposite was prepared by depositing NZVI (Nano Zero Valent Iron, Fe0) over binary GO-CS in seven different compositions for its best optimisation in the solar-light-promoted degradation of RhB. NC (Nano Composite) was characterised by SEM demonstrating their surface morphology. Further characterisation and properties of NC were also studied using XRD, FT-IR, VSM and BET and EDS techniques. The efficacy of the NC was investigated for the removal of RhB in comparison to binary GO-CS and bare NZVI. GCNI 1:1:3 was found to be the best suitable photocatalyst showing synergistic effect in the photodegradation of RhB under given conditions of pH, concentration and time. The mechanism of dye removal and degradation was further discovered by UV-VIS and mass spectroscopy techniques. FT-IR and XRD results of fresh and treated GCNI successively corroborated the mechanism. The sorption kinetics of RhB on to GCNI was found to be described by the pseudo-second-order kinetic equation. The parameters such as dye concentration, pH and the reaction time are varied to understand the effective removal of RhB in wastewater. The outcomes exhibited the highly efficient; up to 99.4% of dye removal, easy magnetic separation of photocatalyst, excellent reusability up-to 87.5% till six consecutive cycles, synergistic effect in adsorption and photo-degradation of dye.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.283
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2021
Admission routes1
Has abstractyes

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