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Record W7146183353

Ab initio calculations of phonons in LiNbO3

2000· article· en· W7146183353 on OpenAlexfundno aff
K. Parlinski, Z. M. Li, Y. Kawazoe

Bibliographic record

VenueInstitutional Repositories DataBase (IRDB) · 2000
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPhotorefractive and Nonlinear Optics
Canadian institutionsnot available
FundersDivision of Materials ResearchNuclear PhysicsNatural Sciences and Engineering Research Council of Canada
KeywordsPhononSoft modesFerroelectricityAb initioDielectricAb initio quantum chemistry methodsNiobiumIonPhase (matter)
DOInot available

Abstract

fetched live from OpenAlex

Using the ab initio method within the local-density approximation with ultrasoft pseudopotentials and plane-wave basis, calculating the Hellmann-Feynman forces and applying the direct method, the phonondispersion relations for ferroelectric and paraelectric rhombohedral phases of LiNbO 3 crystal have been derived.The calculated phonon frequencies for the ferroelectric phase at the point are compared with Raman, infrared, and neutron-scattering measurements, and they agree very well.The phonon frequencies at the Z, L, and F high-symmetry points are also calculated.It is disclosed that the force constants involving lithium ions are an order of magnitude smaller than the force constants between niobium and oxygen ions.As a consequence, the lithium ions do not contribute to high-frequency optical vibrations.In the paraelectric phase the phonon-dispersion curves show a soft branch with the soft mode of symmetry A 2u at the point.This soft mode leads to the observed paraelectric-ferroelectric phase transition.The LO/TO splitting is considered by assuming formal values of ionic charges, and by fitting the longitudinal infrared active modes to the experimental data.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.644
Threshold uncertainty score0.757

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.272
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2000
Admission routes1
Has abstractyes

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