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Record W3001360969 · doi:10.1002/ese3.625

A novel method to evaluate cleaning quality of oil in shale using pyrolysis pyrogram

2020· article· en· W3001360969 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEnergy Science & Engineering · 2020
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of Alberta
FundersNational Natural Science Foundation of China
KeywordsPetrophysicsOil shaleKerogenPetroleum engineeringHydrocarbonPyrolysisMatrix (chemical analysis)Shale oilResidual oilOrganic matterTight oilEnvironmental scienceProcess engineeringPulp and paper industryGeologyChemistrySource rockPorosityChromatographyWaste managementGeotechnical engineeringEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Complete and thorough core cleaning is a critical prerequisite for the precise measurements of most rock's petrophysical parameters. In shale, the oil cleaning process, aimed to remove the volatile hydrocarbons, is often complicated by the requirement for intact solid organic. Evaluation of shale's cleaning methods needs to take structural integrity of organic matrix into account but neglected in the existing researches. Here, we develop a novel evaluation method using a modified ESH (extended slow heating) pyrolysis cycle, which starts at a lower initial temperature of 150°C for 10 minutes and then slowly increases to 650°C by 10°C/min. Hydrocarbons on the ESH pyrogram were divided into light free hydrocarbon (S A ), FHR (fluid‐like hydrocarbon, S B ), and solid organic matter (S C ). We propose a set of quantitative evaluation criterions comparing the results of pyrograms, for different types of the hydrocarbons, at different cleaning conditions. We showed that a modified pyrogram achieves complete cleaning with S A and S B removed while S C remains almost intact. The modified pyrogram achieves complete removal of FHR in the second stage of pyrogram, while earlier researches often report residual FHR. The introduced method improves the accuracy in the identification of production potential in kerogen‐rich shale reservoirs up to about 3% of the total pore volume. Further, the new approach allows a quantitative assessment for the cleaning quality without altering the sample's organic matrix. Future studies on the petrophysical properties of the hydrocarbon‐bearing reservoir rocks may benefit from the thorough hydrocarbon removal achieved through the modified pyrogram methods proposed in this study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.553
Threshold uncertainty score0.755

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.004
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.052
GPT teacher head0.315
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it