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Record W4311351511 · doi:10.3390/su142416666

Biogenic Production of Thiosulfate from Organic and Inorganic Sulfur Substrates for Application to Gold Leaching

2022· article· en· W4311351511 on OpenAlexafffund
James McNeice, Harshit Mahandra, Ahmad Ghahreman

Bibliographic record

VenueSustainability · 2022
Typearticle
Languageen
FieldEngineering
TopicMetal Extraction and Bioleaching
Canadian institutionsQueen's University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsThiosulfateChemistrySulfurSulfideSodium thiosulfateReagentBioleachingLeaching (pedology)Sulfide mineralsSodium sulfideInorganic chemistryHydrogen sulfideTetrathionateEnvironmental chemistryCopperOrganic chemistryGeology

Abstract

fetched live from OpenAlex

Gold mining and processing is an activity with large environmental impact due to the low concentration of gold in ore deposits and chemical resistance to most chemicals. Over 75% of gold is leached from ores using cyanide, however less toxic lixiviants have been proposed in the literature. Thiosulfate is one of these alternative reagents, but high reagent consumption has slowed acceptance in mining operations. Reducing the cost and impact of thiosulfate production is a way to reduce the cost of reagent consumption during leaching. The objective of this study was to evaluate the feasibility of leaching gold from ore with biogenic thiosulfate. Biogenic thiosulfate was produced using a marine methylotroph bacterium from three substrates: sodium sulfide, elemental sulfur, and dimethyl sulfide for application in bioleaching. The different substrates were evaluated to determine conversion efficiency from the sulfur source to biogenic thiosulfate and verified by titration and ion chromatography. Optimal conditions for conversion to thiosulfate were determined to be in the range of pH = 7–8, 25–30 °C, with sodium sulfide as a substrate in a sealed system to prevent sulfide from escaping as hydrogen sulfide gas. An oxide gold ore with a grade of 4.02 g/t was selected as a gold source for leaching experiments. The leaching of gold using the biogenic thiosulfate was compared with chemical thiosulfate solutions under experimental conditions of pH = 9.5, 50 mg/L copper, 500 RPM mixing, and 0.1 L/min air. The efficiency of gold bioleaching was measured using flame atomic absorption spectroscopy and fire assay. Gold extraction efficiencies ranging from 20–60% were achieved using the biogenic thiosulfate, and 27–77% with sodium thiosulfate solutions, respectively. It was concluded that the sodium sulfide substrate was best for producing higher biogenic thiosulfate concentrations and leaching efficiency.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.231
Threshold uncertainty score0.452

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.225
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2022
Admission routes2
Has abstractyes

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