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Impacts of Refining Partially Upgraded Bitumen: Vacuum Gas Oil Hydrotreating

2024· article· en· W4398776207 on OpenAlexaffabout
Anton Alvarez‐Majmutov, Tingyong Xing, Yi Zhang, Rafał Gieleciak, Mohamed Ali, Jinwen Chen

Bibliographic record

VenueEnergy & Fuels · 2024
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsNatural Resources Canada
Fundersnot available
KeywordsHydrodesulfurizationRefining (metallurgy)AsphaltVacuum distillationPetroleum engineeringFuel oilEnvironmental scienceCoker unitOil refineryMaterials scienceWaste managementChemistryMetallurgyDistillationOrganic chemistryGeologyEngineeringComposite materialSulfur

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide This study investigates the hydrotreating characteristics of the vacuum gas oil (VGO) fraction of partially upgraded bitumen (PUB), an alternative refinery feedstock from Canadian oil sand bitumen with processability requirements that are yet to be understood. Hydrotreating experiments were conducted in a continuous hydroprocessing pilot plant using VGOs from PUB prepared in-house via thermal cracking and solvent deasphalting, as well as VGOs from unprocessed bitumen and light crude oil as points of comparison. Blends of VGOs from PUB and light crude oil were also tested. The VGOs from PUB were higher in sulfur, nitrogen, aromatics and resins combined, and contained olefins. The hydrotreating experiments were designed to determine the working temperature to desulfurize and denitrogenate a given VGO feed to levels that would be acceptable for further processing in a refining scheme with fluid catalytic cracking and/or hydrocracking units. Hydrotreating the VGOs from PUB proved more difficult than the VGOs from unprocessed bitumen and light crude oil, requiring a 5–15 °C rise in reaction temperature with respect to the reference VGOs to reach the desired sulfur (<300 wppm) and nitrogen (<100 wppm) targets. The hydrotreated VGOs from PUB were in general more aromatic than those from the reference VGOs, despite having similar sulfur and nitrogen levels. More naphtha and light gas oil were generated during the hydrotreating of the VGOs from PUB as a result of using higher temperatures. Hydrotreating the VGOs from PUB consumed up to 43% more hydrogen compared to VGO from bitumen and more than double relative to the VGO from light crude oil. These trends also extended to the VGO blends containing VGO from PUB.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.057
Threshold uncertainty score0.634

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.225
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2024
Admission routes2
Has abstractyes

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