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Record W4400012012 · doi:10.5772/intechopen.1005789

Applications of Pulsed Laser Ablation in Li-ion Battery Research

2024· book-chapter· en· W4400012012 on OpenAlex
K. D. Gibson, Dongfang Yang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueIntechOpen eBooks · 2024
Typebook-chapter
Languageen
FieldEngineering
TopicLaser-Ablation Synthesis of Nanoparticles
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsMaterials scienceAblationLaser ablationBattery (electricity)IonLaserOptoelectronicsAerospace engineeringEngineeringOpticsChemistryPhysicsPower (physics)

Abstract

fetched live from OpenAlex

Harnessing pulsed laser ablation processes in the manufacturing of energy storage devices is a new and promising strategy for the facile development of next-generation Li-ion batteries. In laser ablation, a pulsed laser is focused on a material surface such that the transfer of energy causes the removal of localized material via high throughput and environmentally-friendly processing. This chapter will provide a summary of the recent advances in laser ablation technologies for producing Li-ion battery materials and components. In terms of electrode optimization, it will examine the use of pulsed lasers to: (1) generate large specific surface area nanoparticles of active materials or stable integrative anodes; (2) deposit compositionally complex and stoichiometric thin film active materials; (3) create electrode architectures with increased Li-ion diffusion kinetics, enhanced wettability or free space to accommodate Si anode volume expansions, and; (4) remove the superficial inactive or solid electrolyte interface layers from electrode surfaces. It will also investigate the laser ablation of current collectors to produce textures with improved adhesion and the use of pulsed lasers for cutting and structuring solid ceramic electrolyte. Finally, this chapter will discuss the application of laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) for chemical composition analysis of Li-ion batteries throughout their operating cycle.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.745
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.041
GPT teacher head0.292
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it