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Record W4404670421 · doi:10.1116/6.0004093

Following the propagation of erroneous x-ray photoelectron spectroscopy peak fitting through the literature. A genealogical approach

2024· article· en· W4404670421 on OpenAlexaff
Brennen Clark, George H. Major, Joshua W. Pinder, Daniel E. Austin, Donald R. Baer, Mark C. Biesinger, Christopher D. Easton, Sarah L. Harmer, Alberto Herrera‐Gómez, A.E. Hughés, William Skinner, Matthew R. Linford

Bibliographic record

VenueJournal of Vacuum Science & Technology A Vacuum Surfaces and Films · 2024
Typearticle
Languageen
FieldMaterials Science
TopicElectron and X-Ray Spectroscopy Techniques
Canadian institutionsWestern University
Fundersnot available
KeywordsX-ray photoelectron spectroscopyX-rayMaterials sciencePhysicsOpticsNuclear magnetic resonance

Abstract

fetched live from OpenAlex

This study considers how poor x-ray photoelectron spectroscopy (XPS) peak fitting in the scientific literature is both affected by previous precedent and affects future published work. It focuses on a highly cited paper (the “Subject” paper) from a respected journal that contains incorrect S 2p peak fits. This paper was studied in a genealogical fashion vis-à-vis the XPS peak fitting in its “child,” “parent,” “grandparent,” and “great-grandparent” papers. Interestingly, precedents were not followed to a high degree between parent and child papers. However, in many cases, even when the authors of a study did not follow the incorrect precedent that they cited, they still incorrectly fit their data. Thus, not necessarily for good reasons, the effects of poor XPS peak fits on future generations of papers may be less than some experts had expected or feared. In many cases, older papers appear to contain better XPS peak fitting than newer ones.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.083
metaresearch head score (Gemma)0.310
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesMetaresearch, Research integrity
Consensus categoriesnone
DomainCandidate signal: Reproducibility · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.997
Threshold uncertainty score0.441

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0830.310
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0270.017
Science and technology studies0.0030.003
Scholarly communication0.0110.011
Open science0.0030.004
Research integrity0.0030.002
Insufficient payload (model declined to judge)0.0030.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.277
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

Study designObservational
DomainReproducibility
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2024
Admission routes1
Has abstractyes

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