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Record W4405044938 · doi:10.1016/j.wmb.2024.12.001

Assessment of the potential of oily sludge char for removing organics from petroleum refinery wastewater

2024· article· en· W4405044938 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueWaste Management Bulletin · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsImperial Oil (Canada)University of Alberta
Fundersnot available
KeywordsRefineryWaste managementCharOil refineryWastewaterEnvironmental sciencePetroleumPetroleum productPulp and paper industryChemistryEngineeringCoalOrganic chemistry

Abstract

fetched live from OpenAlex

• ZnCl 2 -activated-oily sludge char (SB-Zn-400) has heterogeneous surface supporting multilayer adsorption. • SB-Zn-400 achieved rapid COD removal, reaching equilibrium within 2 h with a 28 % reduction in COD. • >97 % of various organic compounds in PR-WW were effectively removed by SB-Zn-400. • Hydrogen bonding and π-π interactions were the main adsorption mechanism. • Thermal regeneration of SB-Zn-400 allows for reuse, maintaining higher adsorption efficiency compared to pristine-OSC. Oil sludge (OS), a by-product of petroleum refinery (PR) waste, contains various toxic organic and inorganic compounds. Improper handling of OS poses serious environmental risks, highlighting the need for an effective and sustainable solution to mitigate these hazards and transform OS into a valuable product. This study converted OS into char-(OSC), including both pristine-OSC and ZnCl 2 -activated-OSC, for the removal of organic pollutants from refinery wastewater (WW) with a high COD concentration (89,233 mg/L). ZnCl 2 -activated-OSC produced at 400 °C (SB-Zn-400) showed superior adsorption capacity compared to pristine-OSC, due to enhanced oxygen-containing functional groups, crystallinity, thermostability, and superior degradation (OS). The adsorption process demonstrated rapid COD removal, reaching equilibrium within 2 h and achieving a 28 % reduction in COD. The adsorption capacity was found to be 420.5 mg-COD/g-OSC. SB-Zn-400 exhibited heterogeneous surface properties and supported multi-layer adsorption, with hydrogen-bonding and π–π interactions likely adsorption mechanisms. Moreover, the total concentration of organic compounds in PR-WW was >2700 mg/L, and SB-Zn-400 reduced this concentration to 34 mg/L, achieving >98 % removal. Although the adsorption treatment reduced the inorganic parameters of PR-WW, leaching of Mn, Ni, and Zn was observed, likely due to the nature of OS and the ZnCl 2 -activation process. Thermal regeneration of spent SB-Zn-400 allowed the reuse of OSC, with adsorption efficiency remaining higher than that of pristine-OSC, indicating that SB-Zn-400 has potential to be reused. These findings highlight the effectiveness of OSC in treating PR-WW, supporting a circular economy approach to enhance resource efficiency and minimize the environmental impact of OS from PR industries.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.871
Threshold uncertainty score0.996

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.213
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it