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Record W4405756504 · doi:10.1021/acs.est.4c10931

A Novel Organophosphate Ester, Tris(2,4-di<i>tert</i>-butylphenyl) Phosphate, Induced Reproductive Toxicity in Male Zebrafish at Environmentally Relevant Concentrations

2024· article· en· W4405756504 on OpenAlexaff
Yongkang Zhang, Haiyu Qin, Boqun Li, Zichen Yu, Bowen Zu, Ren Kong, Robert J. Letcher, Chunsheng Liu, Bingsheng Zhou

Bibliographic record

VenueEnvironmental Science & Technology · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicEffects and risks of endocrine disrupting chemicals
Canadian institutionsCarleton University
FundersNational Key Research and Development Program of ChinaChina University of GeosciencesNational Natural Science Foundation of China
KeywordsZebrafishSemen qualityToxicityOrganophosphateSpermBiologyReproductive toxicitySperm motilitySpermatogenesisAndrologyMotilityIn vivoEndocrine disruptorChemistryInternal medicineEndocrinologyCell biologyPesticideBiochemistryGeneEcologyGeneticsMedicine

Abstract

fetched live from OpenAlex

Abstract As a novel organophosphate ester (NOPE), tris­(2,4-ditert-butylphenyl) phosphate (TDtBPP) has attracted significant attention due to its unexpectedly high detection in natural environments. However, the ecological toxic effects of environmentally relevant concentrations of TDtBPP in organisms remain entirely unknown. In this study, 1 month old zebrafish were exposed to 0, 50, 500, or 5000 ng/L TDtBPP for 150 days, and the reproductive toxicity in male fish was evaluated. Results demonstrated that TDtBPP exposure significantly inhibited the maturation of spermatozoa and thus decreased spermatogenesis. Furthermore, abnormal sperm morphology and decreased sperm motility were also observed. The decrease in sperm quantity and quality eventually resulted in the declining fecundity. Moreover, TDtBPP exposure downregulated the expression of hsd3b1 in vivo and in vitro and subsequently inhibited the synthesis of androgens in zebrafish testes and Leydig cells. This inhibition of androgen synthesis appeared to be responsible for the observed reproductive toxicity in male fish. Molecular docking and dual-luciferase reporter gene experiments elucidated that TDtBPP inhibited the promotion of vitamin D on hsd3b1 transcription by the vitamin D receptor and thus downregulated the expression of hsd3b1. Our findings provide first time evidence that TDtBPP poses a risk to male fish reproduction at environmentally relevant levels.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.267
Teacher spread0.260 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2024
Admission routes1
Has abstractyes

Explore more

Same venueEnvironmental Science & Technology→Same topicEffects and risks of endocrine disrupting chemicals→French-language works237,207→