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Cosmic Ray Irradiation of Interstellar Ices on Sulfur-Rich Grains: A Possible Source of Sulfur-Bearing Molecules

2025· article· en· W4410163803 on OpenAlexfundno aff
Duncan V. Mifsud, Z. Kaňuchová, Olivier Auriacombe, Péter Herczku, D. Qasim, Sándor Kovács, R. Rácz, B. Sulik, Zoltán Juhász, I. Rajta, I. Vajda, S. Biri, R. W. McCullough, S. Ioppolo, U. Raut, N. J. Mason

Bibliographic record

VenueACS Earth and Space Chemistry · 2025
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAstrophysics and Star Formation Studies
Canadian institutionsnot available
FundersEuropean Regional Development FundNemzeti Kutatási Fejlesztési és Innovációs HivatalQueen's UniversityUniversity of KentNational Research FoundationSpace Telescope Science InstituteEuropean Cooperation in Science and TechnologyDanmarks GrundforskningsfondHorizon 2020 Framework ProgrammeQueen's University BelfastMagyar Tudományos AkadémiaRoyal SocietyHungarian Research Network
KeywordsSulfurCosmic rayAstrobiologyIrradiationBearing (navigation)MoleculeInterstellar mediumMaterials scienceRadiochemistryPhysicsChemistryAstrophysicsAstronomyNuclear physicsMetallurgyOrganic chemistryGalaxy

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide The major reservoir of sulfur in dense interstellar clouds is still largely unknown, although a growing body of evidence suggests that it may exist in a refractory form (i.e., as minerals or allotropes of the element). Therefore, it is possible that the irradiation of sulfur-free interstellar ices on top of sulfur-rich refractory grain components by cosmic rays or stellar winds may result in the formation of simple inorganic sulfur molecules that could be readily detected by ground- or space-borne telescopes. In this study, we have irradiated neat ices of O 2, CO, CO 2, and H 2 O on top of layers of allotropic sulfur at 20 K using 1 MeV He + ions as a mimic of space radiation. Experiments with CO 2 and H 2 O ices were also repeated at 70 K to provide data obtained under conditions more relevant to icy bodies in the outer solar system for comparative purposes. We have found qualitative mid-infrared spectroscopic evidence for the synthesis of SO 2, CS 2, OCS, and H 2 SO 4 hydrates, but not H 2 S, in our experiments and have quantified the efficiency of their formation by calculating the G -value (i.e., the number of molecules formed per 100 eV of energy deposited) for each ice-refractory system. Overall, SO 2 and CS 2 are the most commonly observed products in our experiments, although the highest G -value was that for H 2 SO 4 hydrates formed as a result of the irradiation of H 2 O ice on top of sulfur at 70 K. An important outcome of our study is that our experimental results are consistent with recent observational surveys that suggest SO 2 formation in interstellar ices proceeds primarily via an “energetic” route involving radiolytic processes, while OCS forms as a result of “nonenergetic” processes such as atom or radical addition reactions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.152
Threshold uncertainty score0.447

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.212
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes1
Has abstractyes

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