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Impact of below-freezing air temperatures on the formation and stability of seawater-crude oil emulsion

2025· article· en· W4410855565 on OpenAlexaff
Jianyun Li, Wen Ji, Roger C. Prince, Kenneth Lee, W. Scott Pegau, Michel C. Boufadel

Bibliographic record

VenueMarine Pollution Bulletin · 2025
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsGreenfield Research (Canada)
FundersOil Spill Recovery Institute
KeywordsEmulsionSeawaterCrude oilEnvironmental scienceChemistryPetroleum engineeringOceanographyGeologyOrganic chemistry

Abstract

fetched live from OpenAlex

The formation of 'seawater-in-oil' emulsions reduces the effectiveness of current oil spill response operations such as the physical recovery of oil with skimmers, or oil dispersion with chemical dispersants, due to increases in volume and viscosity. This becomes even more acute in cold regions because of the potential for below-freezing temperatures and floating ice. Low temperatures increase oil viscosity and can freeze entrained water droplets, potentially inhibiting the formation of new emulsions while stabilizing any that have already formed. Existing works on emulsion behavior at near-freezing temperatures may have underestimated the impact of below-freezing air temperatures, common in polar regions, on the formation and stability of seawater-in-oil emulsion. To address this issue, we investigated the behavior of emulsions exposed to below-freezing air temperatures (-20 °C), studying oils with different asphaltene contents. Higher asphaltene content (18 wt%) was correlated with increased emulsion stability, but emulsions that experienced freezing air temperatures were more prone to break during thawing. After -20 °C treatment, Hibernia emulsions lost >50 % of their entrained water, while Alaska North Slope emulsions lost >25 %. Samples kept at 20 °C lost far less. Emulsions exposed to significantly sub-zero temperatures in Polar regions are thus likely to break when they thaw, which will impact oil spill response.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.238
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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